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The Atomistic Perspective of Nanoscale Laser Ablation

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Ultrafast Laser Nanostructuring

Part of the book series: Springer Series in Optical Sciences ((SSOS,volume 239))

Abstract

Materials irradiated by ultrashort laser pulses can undergo a variety of surface relief and structural modifications due to melting, spallation, and ablation processes. The possibility of instant and localized energy deposition into materials makes the short laser pulses a perspective tool in precise material modifications under controlled conditions. Thus, with certain laser irradiation parameters, the absorbed energy can trigger one or several laser-induced phase transition processes in the solid leading to material ejection, generation of subsurface voids, or nanostructures growth on the surface. The resulting material modifications can change its topographical, morphological, magnetic, and optical properties. While the ablation and spallation processes were utilized in laser welding and drilling technology, the functionalized surfaces have found a number of applications in micro-optics, waveguides, Raman spectroscopy, and biosensors. Generation of material modifications in a designed way, however, requires a detailed understanding of the dynamics of fast, nonequilibrium, and interrelated laser-induced processes at nanoscale. In this work, a combined particle-based mesoscopic numerical approach suitable for the investigation of ablation and nanostructuring mechanism of solids on the experimental scale is proposed. The combined model is applied to investigate the laser-induced processes and their dependences on the surrounding media and laser irradiation parameters: wavelength, pulse duration, and fluence. Good agreement between the modeling and the experimental results justifies the proposed approach as a powerful numerical tool revealing the fundamental physics of the underlying the ablation and nanostructuring processes. This will pave the way toward predesigned topography for functionalized surfaces on the nanoscales.

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Acknowledgments

We acknowledge the financial support of the Deutsche Forschungsgemeinschaft projects RE1141/14-2, IH 17/18-2, GA465/15-2, and IV122/4-1 and RFBR Project Number 20-02-00861. The MD-TTM calculations were performed at Lichtenberg Super Computer Facility TU-Darmstadt (Germany). Some simulations were executed on the high-performance cluster “Elwetritsch” through the projects TopNano and Mulan at the TU Kaiserslautern, which is a part of the “Alliance of High Performance Computing Rheinland-Pfalz.” P.N.T. and B.R. kindly acknowledge the support of Regionales Hochschulrechenzentrum Kaiserslautern.

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Authors and Affiliations

  1. P.N. Lebedev Physical Institute, Moscow, Russia

    Dmitry S. Ivanov, Sergey I. Kudryashov & Irina N. Zavestovskaya

  2. Department of Physics and Research Center OPTIMAS, Technical University of Kaiserslautern, Kaiserslautern, Germany

    Pavel N. Terekhin & Baerbel Rethfeld

  3. Institute of Engineering Physics for Biomedicine (PhysBio), Moscow, Russia

    Sergey M. Klimentov, Andrei V. Kabashin & Irina N. Zavestovskaya

  4. LP3, Aix Marseille Univ, CNRS, LP3, Campus de Luminy, Marseille, France

    Andrei V. Kabashin

  5. Institute of Physics and Center for Interdisciplinary Nanostructure Science and Technology (CINSaT), University of Kassel, Kassel, Germany

    Martin E. Garcia

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    Razvan Stoian

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Ivanov, D.S. et al. (2023). The Atomistic Perspective of Nanoscale Laser Ablation. In: Stoian, R., Bonse, J. (eds) Ultrafast Laser Nanostructuring. Springer Series in Optical Sciences, vol 239. Springer, Cham. https://doi.org/10.1007/978-3-031-14752-4_2

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