Abstract
The intensity-dependent transmission of picosecond ruby laser pulses of different duration through methanolic and ethanolic solutions of rhodamine B and rhodamine 6G is analysed. The transmission is affected by S0-S n two-photon absorption, by stimulated emission at the pump-laser frequency, by amplified spontaneous emission and by excited-state absorption. Various parameters involving the two-photon absorption dynamics are determined by comparing experiments with numerical simulations.
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F. P. SCHÄFER and W. SCHMIDT,IEEE J. Quantum Electron. QE-2 (1966) 357.
D. J. BRADLEY, M. H. R. HUTCHINSON and H. KOETSER,Proc. R. Soc. A329 (1972) 105.
J. P. HERMANN and J. DUCUING,Opt. Commun. 6 (1972) 101.
E. B. ASLANIDI and E. A. TIKHONOV,Opt. Spectrosc. 37 (1974) 446.
J. KRASINSKI, W. MAJEWSKI and M. GLÓDŹ,Opt. Commun. 14 (1975) 187.
B. FOUCAULT and J. P. HERMANN,ibid. 15 (1975) 412.
L. PARMA and N. OMENETTO,Chem. Phys. Lett. 54 (1978) 541.
J. A. GIORDMAINE, P. M. RENTZEPIS, S. L. SHAPIRO and K. W. WECHT,Appl. Phys. Lett. 11 (1967) 216.
W. RAPP and B. GRONAU,Chem. Phys. Lett. 8 (1971) 529.
A. N. RUBINOV, M. C. RICHARDSON, K. SALA and A. J. ALCOCK,Appl. Phys. Lett. 27 (1975) 358.
D. J. BRADLEY, T. MORROW and M. S. PETTY,Opt. Commun. 6 (1972) 394.
R. PARETTI and P. RANSON,ibid. 3 (1971) 62.
D. J. BRADLEY, M. H. R. HUTCHINSON, H. KOETSER, T. MORROW, G. H. C. NEW and M. S. PETTY,Proc. R. Soc. A328 (1972) 97.
S. MORY, D. LEUPOLD and R. KÖNIG,Opt. Commun. 6 (1972) 394.
J. HERRMANN, M. PALME and K. E. SÜSSE,Opt. Quantum Electron. 10 (1978) 195.
S. J. STRICKLER and R. A. BERG,J. Chem. Phys. 37 (1962) 814.
D. RICARD and J. DUCUING,J. Chem. Phys. 62 (1975) 3616.
A. SEILMEIER, P. O. J. SCHERER and W. KAISER,Chem. Phys. Lett. 105 (1984) 140.
D. N. DEMPSTER,J. Photochem. 2 (1973) 343.
B. G. HUTH, G. I. FARMER and M. R. KAGEN,J. Appl. Phys. 40 (1969) 5145.
W. BLAU, W. DANKESREITER and A. PENZKOFER,Chem. Phys. 85 (1984) 473.
A. PENZKOFER and P. SPERBER,ibid. 88 (1984) 309.
N. I. KUNAVIN, R. N. NURRUKHAMETOV and G. T. KHACHATUROVA,Sov. J. Appl. Spectrosc. 26 (1977) 735.
Y. LU and A. PENZKOFER,Chem. Phys. 107 (1986) 175.
A. PENZKOFER and Y. LU,ibid. 103 (1986) 399.
W. M. McCLAIN,Acc. Chem. Res. 7 (1974) 129.
A. PENZKOFER and W. FALKENSTEIN,Chem. Phys. Lett. 44 (1976) 547.
A. PENZKOFER and W. BLAU,Opt. Quantum Electron. 15 (1983) 325.
Th. FÖRSTER,Z. Naturforsch. 4a (1949) 321.
K. H. DREXHAGE,Laser Focus 9(3) (1973) 35.
O. G. PETERSON, J. P. WEBB, W. C. McCOLGIN and J. E. EBERLY,J. Appl. Phys. 42 (1971) 1917.
M. J. WEBER and M. BASS,IEEE J. Quantum Electron. 5 (1969) 175.
B. B. SNAVELY, in ‘Photophysics of Aromatic Molecules’, edited by J. B. Birks (Wiley, London, 1973) p. 239.
P. R. HAMMOND,IEEE J. Quantum Electron. QE-15 (1979) 624.
Idem, ibid. QE-16 (1980) 1157.
J. WIEDMANN and A. PENZKOFER,Nuovo Cimento 63B (1981) 459.
W. BLAU and A. PENZKOFER,Opt. Commun. 36 (1981) 419.
A. PENZKOFER,Opto-Electronics 6 (1974) 87.
A. PENZKOFER and W. FALKENSTEIN,Opt. Quantum Electron. 10 (1978) 399.
W. FALKENSTEIN, A. PENZKOFER and W. KAISER,Opt. Commun. 27 (1978) 151.
M. D. GALANIN and S. A. TSCHISCHKOWA,Kratk. Soobshch. Fiz. 4 (1971) 35.
I. KAPLAN and J. JORTNER,J. Chem. Phys. 32 (1978) 381.
A. V. ARISTOV and Yu. S. MASLYUKOV,Opt. Spectrosc. 41 (1976) 141.
D. W. PHILLION,Appl. Phys. Lett. 27 (1975) 85.
K. A. SELANGER, J. FALNES and T. SIKKELAND,J. Phys. Chem. 81 (1977) 1960.
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Sperber, P., Penzkofer, A. S0-S n two-photon absorption dynamics of rhodamine dyes. Opt Quant Electron 18, 381–401 (1986). https://doi.org/10.1007/BF02032565
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DOI: https://doi.org/10.1007/BF02032565