Skip to main content
Log in

S0-S n two-photon absorption dynamics of rhodamine dyes

  • Published:
Optical and Quantum Electronics Aims and scope Submit manuscript

Abstract

The intensity-dependent transmission of picosecond ruby laser pulses of different duration through methanolic and ethanolic solutions of rhodamine B and rhodamine 6G is analysed. The transmission is affected by S0-S n two-photon absorption, by stimulated emission at the pump-laser frequency, by amplified spontaneous emission and by excited-state absorption. Various parameters involving the two-photon absorption dynamics are determined by comparing experiments with numerical simulations.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. F. P. SCHÄFER and W. SCHMIDT,IEEE J. Quantum Electron. QE-2 (1966) 357.

    Article  Google Scholar 

  2. D. J. BRADLEY, M. H. R. HUTCHINSON and H. KOETSER,Proc. R. Soc. A329 (1972) 105.

    Google Scholar 

  3. J. P. HERMANN and J. DUCUING,Opt. Commun. 6 (1972) 101.

    Article  Google Scholar 

  4. E. B. ASLANIDI and E. A. TIKHONOV,Opt. Spectrosc. 37 (1974) 446.

    Google Scholar 

  5. J. KRASINSKI, W. MAJEWSKI and M. GLÓDŹ,Opt. Commun. 14 (1975) 187.

    Article  Google Scholar 

  6. B. FOUCAULT and J. P. HERMANN,ibid. 15 (1975) 412.

    Article  Google Scholar 

  7. L. PARMA and N. OMENETTO,Chem. Phys. Lett. 54 (1978) 541.

    Article  Google Scholar 

  8. J. A. GIORDMAINE, P. M. RENTZEPIS, S. L. SHAPIRO and K. W. WECHT,Appl. Phys. Lett. 11 (1967) 216.

    Article  Google Scholar 

  9. W. RAPP and B. GRONAU,Chem. Phys. Lett. 8 (1971) 529.

    Article  Google Scholar 

  10. A. N. RUBINOV, M. C. RICHARDSON, K. SALA and A. J. ALCOCK,Appl. Phys. Lett. 27 (1975) 358.

    Article  Google Scholar 

  11. D. J. BRADLEY, T. MORROW and M. S. PETTY,Opt. Commun. 6 (1972) 394.

    Article  Google Scholar 

  12. R. PARETTI and P. RANSON,ibid. 3 (1971) 62.

    Article  Google Scholar 

  13. D. J. BRADLEY, M. H. R. HUTCHINSON, H. KOETSER, T. MORROW, G. H. C. NEW and M. S. PETTY,Proc. R. Soc. A328 (1972) 97.

    Google Scholar 

  14. S. MORY, D. LEUPOLD and R. KÖNIG,Opt. Commun. 6 (1972) 394.

    Article  Google Scholar 

  15. J. HERRMANN, M. PALME and K. E. SÜSSE,Opt. Quantum Electron. 10 (1978) 195.

    Article  Google Scholar 

  16. S. J. STRICKLER and R. A. BERG,J. Chem. Phys. 37 (1962) 814.

    Article  Google Scholar 

  17. D. RICARD and J. DUCUING,J. Chem. Phys. 62 (1975) 3616.

    Article  Google Scholar 

  18. A. SEILMEIER, P. O. J. SCHERER and W. KAISER,Chem. Phys. Lett. 105 (1984) 140.

    Article  Google Scholar 

  19. D. N. DEMPSTER,J. Photochem. 2 (1973) 343.

    Article  Google Scholar 

  20. B. G. HUTH, G. I. FARMER and M. R. KAGEN,J. Appl. Phys. 40 (1969) 5145.

    Article  Google Scholar 

  21. W. BLAU, W. DANKESREITER and A. PENZKOFER,Chem. Phys. 85 (1984) 473.

    Article  Google Scholar 

  22. A. PENZKOFER and P. SPERBER,ibid. 88 (1984) 309.

    Article  Google Scholar 

  23. N. I. KUNAVIN, R. N. NURRUKHAMETOV and G. T. KHACHATUROVA,Sov. J. Appl. Spectrosc. 26 (1977) 735.

    Article  Google Scholar 

  24. Y. LU and A. PENZKOFER,Chem. Phys. 107 (1986) 175.

    Article  Google Scholar 

  25. A. PENZKOFER and Y. LU,ibid. 103 (1986) 399.

    Article  Google Scholar 

  26. W. M. McCLAIN,Acc. Chem. Res. 7 (1974) 129.

    Article  Google Scholar 

  27. A. PENZKOFER and W. FALKENSTEIN,Chem. Phys. Lett. 44 (1976) 547.

    Article  Google Scholar 

  28. A. PENZKOFER and W. BLAU,Opt. Quantum Electron. 15 (1983) 325.

    Article  Google Scholar 

  29. Th. FÖRSTER,Z. Naturforsch. 4a (1949) 321.

    Google Scholar 

  30. K. H. DREXHAGE,Laser Focus 9(3) (1973) 35.

    Google Scholar 

  31. O. G. PETERSON, J. P. WEBB, W. C. McCOLGIN and J. E. EBERLY,J. Appl. Phys. 42 (1971) 1917.

    Article  Google Scholar 

  32. M. J. WEBER and M. BASS,IEEE J. Quantum Electron. 5 (1969) 175.

    Article  Google Scholar 

  33. B. B. SNAVELY, in ‘Photophysics of Aromatic Molecules’, edited by J. B. Birks (Wiley, London, 1973) p. 239.

    Google Scholar 

  34. P. R. HAMMOND,IEEE J. Quantum Electron. QE-15 (1979) 624.

    Article  Google Scholar 

  35. Idem, ibid. QE-16 (1980) 1157.

    Article  Google Scholar 

  36. J. WIEDMANN and A. PENZKOFER,Nuovo Cimento 63B (1981) 459.

    Google Scholar 

  37. W. BLAU and A. PENZKOFER,Opt. Commun. 36 (1981) 419.

    Article  Google Scholar 

  38. A. PENZKOFER,Opto-Electronics 6 (1974) 87.

    Article  Google Scholar 

  39. A. PENZKOFER and W. FALKENSTEIN,Opt. Quantum Electron. 10 (1978) 399.

    Article  Google Scholar 

  40. W. FALKENSTEIN, A. PENZKOFER and W. KAISER,Opt. Commun. 27 (1978) 151.

    Article  Google Scholar 

  41. M. D. GALANIN and S. A. TSCHISCHKOWA,Kratk. Soobshch. Fiz. 4 (1971) 35.

    Google Scholar 

  42. I. KAPLAN and J. JORTNER,J. Chem. Phys. 32 (1978) 381.

    Article  Google Scholar 

  43. A. V. ARISTOV and Yu. S. MASLYUKOV,Opt. Spectrosc. 41 (1976) 141.

    Google Scholar 

  44. D. W. PHILLION,Appl. Phys. Lett. 27 (1975) 85.

    Article  Google Scholar 

  45. K. A. SELANGER, J. FALNES and T. SIKKELAND,J. Phys. Chem. 81 (1977) 1960.

    Article  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Sperber, P., Penzkofer, A. S0-S n two-photon absorption dynamics of rhodamine dyes. Opt Quant Electron 18, 381–401 (1986). https://doi.org/10.1007/BF02032565

Download citation

  • Received:

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1007/BF02032565

Keywords

Navigation