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Rapid method for alpha counting with extractive scintillator and pulse shape analysis

  • Actinides in Environment and Waste Disposal Problem
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Abstract

A rapid method for alpha counting with liquid scintillation is presented. The interference of beta and gamma radiation with the determination of alpha emitting nuclides by liquid scintillation counting was examined. In extractive scintillator cocktail, TOPO-PPO-naphthalene-toluene has been developed for transferring actinide elements into organic scintillator and separating the undesirable materials as well as most beta emitters. Pulse Shape Analysis (PSA) was applied for the discrimination of beta radiation. The influence of cocktail composition on PSA has been studied and compared with that of the commercial cocktail. An analytical procedure was suggested for the rapid determination of actinide elements U, Pu, Am and Cm in the nuclear fuel cycle or in environmental samples.

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References

  1. D. HORROCKS, Rev. Sci. Instrum., 35 (1964) 334.

    Google Scholar 

  2. D. L. HORROCKS, M. H. STUDIER, Anal. Chem., 36 (1964) 2077.

    Google Scholar 

  3. K. FLYNN, L. GLENDENIN, E. STEINSERS, P. WRISHT, Nucl. Instrum. Methods, 27 (1964) 13.

    Google Scholar 

  4. H. IHLE, M. KARAYANNIS, P. MRRENHOFF, Liquid Scintillation Counting of Alpha Emitters, in: Proc. Sympos. on Radioisotope Sample Measurement Techniques, IAEA, Vienna, 1965, p. 483.

    Google Scholar 

  5. A. LINDERBAUM, C. JUDD, Radiation Res., 37 (1969) 131.

    PubMed  Google Scholar 

  6. W. J. McDOWELL, Liquid Scintillation Counting Technique for the Higher Actinides, in: Organic S cin tillator and Liquid Scintillation Counting, D. L. HORROCKS and C. T. PENG (Eds), Academic Press, New York, 1971, p. 937.

    Google Scholar 

  7. W. J. McDOWELL, C. F. COLEMAN, Combined Solvent Extraction-Liquid Scintillation Method for Radioassay of Alpha Emitters, in: Proc. Intern. Solvent Extraction Conference, London, 1974.

  8. J. H. THORNGATE, W. J. McDOWELL, D. J. CHRISTIAN, Health Phys., 27 (1974) 132.

    PubMed  Google Scholar 

  9. J. W. McKLVEEN, W. R. JOHNSON, Health Phys., 28 (1975) 5.

    PubMed  Google Scholar 

  10. J. W. McKLVEEN, W. J. McDOWELL, Nuclear Technol., 28 (1976) 159.

    Google Scholar 

  11. W. J. McDOWELL, Alpha Liquid Scintillation Counting; Past, Present and Future, in: Liquid Scintillation Counting: Recent Applications and Development, C. T. PENS, D. L. HORROCKS and E. L. ALPEN (Eds), Academic Press, New York, 1980), p. 315.

    Google Scholar 

  12. Y. BABA, J. Radioanal. Chem. 79, (1983) 83.

    Google Scholar 

  13. J. W. McKLVEEN, W. J. McDOWELL, Nucl. Instrum. Methods Phys. Res., Sect. A, 223 (1983) 372.

    Google Scholar 

  14. J. W. McDOWELL, G. N. CASE, Separation and Methods for Alpha Assay by Liquid Scintillation, in: Chemical Aspects of Nuclear Methods of Analysis, IAEA-TECDOC-350, Vienna, 1985, p. 33.

  15. W. J. McDOWELL, Alpha Counting and Spectrometry Using Liquid Scin tillation Method, Report NAS-NS-3116, 1986.

  16. J. H. THORNGATE, W. J. McDOWELL, D. J. CHRISTIAN, Health Phys., 27 (1974) 123.

    PubMed  Google Scholar 

  17. J. H. THORNGATE, D. J. CHRISTIAN, Health Phys., 33 (1977) 443.

    PubMed  Google Scholar 

  18. J. H. THORNGATE, Health Phys., 34 (1978) 103.

    PubMed  Google Scholar 

  19. L. K. B. WALLACE, 1219 Spectra Master, Product Information Package, 1987.

  20. L. M. BOLLINGER, G. E. THOMAS, Rev. Sci. Instr., 32 (1964) 1044.

    Google Scholar 

  21. D. L. HORROCKS, Application of Liquid Scintillation Counting, Academic Press, New York, 1974.

    Google Scholar 

  22. M. BENEDICT, T. H. PIGFORD, H. W. LEVI, Nuclear Chemical Engineering, McGraw-Hill, London, 1981.

    Google Scholar 

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Dazhu, Y., Yongjun, Z. & Möbius, S. Rapid method for alpha counting with extractive scintillator and pulse shape analysis. Journal of Radioanalytical and Nuclear Chemistry, Articles 147, 177–189 (1991). https://doi.org/10.1007/BF02039579

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  • DOI: https://doi.org/10.1007/BF02039579

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