Abstract
We present systematic low temperature in situ119Sn Mössbauer effect (ME) studies in vapor quenched amorphous Mn x Sn1−x (0.09<x<0.95) alloys between 150 and 4.2 K. It is shown that the magnetic behavior of the system is correctly displayed by the transferred magnetic hyperfine (hf) interactions detected at the119Sn site. Combining the results of the concentration dependence of the transferred magnetic hf field and the ordering temperature with recent ac-magnetic susceptibility data reported on this system, a complete magnetic phase diagram is proposed. The effect of an external magnetic field (up to about 3 T) on the spin correlations in the spin-glass state is also discussed.
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Values of the magnetic ordering temperature,T o, deduced from119Sn ME measurements are slightly higher than those obtained fromX ac method [9]. This is known to be related to the dynamical nature (relaxation effects) of the SG freezing.
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Drago, V., Saitovitch, E.B. & Abd-Elmeguid, M.M. Mössbauer studies of the magnetic behavior of amorphous Mn x Sn1−x alloys. Hyperfine Interact 51, 1061–1068 (1989). https://doi.org/10.1007/BF02407826
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DOI: https://doi.org/10.1007/BF02407826