Abstract
A theoretical model is presented to explain the spin gap observed for CaV4O9. The lattice structure is the regularly 1/5-depleted square lattice, where a plaquette formed byJ p is connected to the neighboring four plaquettes byJ d . BothJ p andJ p are antiferromagnetic. At isotropic coupling (J p =J d ) the ground state shows the Néel ordering, but is close vicinity of the quantum critical point to the plaquette resonating-valence-bond (PRVB) state. We show that a small frustrating next-nearest-neighbor interaction can drive the system into the PRVB state and thus explain a large spin gap compatible with experiments.
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Kontani, H., Troyer, M., Ueda, K. et al. Plaquette resonating-valence-bond ground state of CaV4O9 . Czech J Phys 46 (Suppl 4), 1903–1904 (1996). https://doi.org/10.1007/BF02570943
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DOI: https://doi.org/10.1007/BF02570943