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Structures and Biological Effects pp 41–113Cite as

Recent aspects of the structure and reactivity of cyclophosphazenes

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Part of the book series: Structure and Bonding ((STRUCTURE,volume 81))

Abstract

This review describes the reactivity and structural aspects of cyclophosphazenes. The reactions of halogenocyclophosphazenes with a variety of monofunctional and difunctional reagents are described. The mechanisms of the reactions involved are discussed in light of kinetic evidence and product analysis. Reactions involving main-group and transition-metal reagents and halogenocyclophosphazenes are also described. The chemistry of hydridophosphazenes containing a P-H bond is described in more detail. Some of the rearrangement reactions including cis-trans isomerism and tautomerism which are common to some cyclophosphazene derivatives have been discussed. The coordination chemistry involving cyclophosphazenes as ligands via endocyclic and/or exocyclic coordination sites resulting in several types of derivatives including metallocenyl cyclophosphazenes, metal clusters and carboranyl cyclophosphazenes has been critically evaluated. The structural aspects of cyclophosphazenes have been reviewed with particular emphasis on multinuclear NMR and single crystal X-ray methods. Bond angle-bond length variations in X-ray structures of cyclophosphazenes have been explained based on the theories of bonding prevalent in these molecules.

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    V. Chandrasekhar & K. R. Justin Thomas

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Chandrasekhar, V., Justin Thomas, K.R. (1993). Recent aspects of the structure and reactivity of cyclophosphazenes. In: Structures and Biological Effects. Structure and Bonding, vol 81. Springer, Berlin, Heidelberg. https://doi.org/10.1007/BFb0036817

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