Abstract
An electrochemical technique is used to study local mass transfer coefficients on surfaces of inclined enclosures over the range 1.1×104 < RaH < 1.4×1010 for a nominal Schmidt number of 2280. Scaling with gcosθ instead of g in the Rayleigh number correlates the data well at low angles of inclination; however, as either the aspect ratio or the angle of inclination increase, the longitudinal density stratification causes the data to deviate from a power law scaling.
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Notes
We assume that for the fluid of interest, density decreases with temperature
Abbreviations
- ΔCi::
-
Concentration difference for species i(mol/l)
- Di::
-
Diffusion coefficient of species i (m2/s)
- F::
-
Faraday’s constant (96,487 C/g mol)
- g::
-
Acceleration due to gravity (9.8 m/s2)
- h::
-
Mass transfer coefficient
- H::
-
Thickness of fluid layer between electrodes (m)
- i::
-
Species of interest (copper ions)
- I::
-
Current (A)
- L::
-
Length of cathode surface (m)
- ni::
-
Valence of transferred ion
- Pr::
-
Prandtl number (ν/α)
- RaL::
-
Mass transfer Rayleigh number based on cathode length [g(ρbulk-ρc) L3/ρν Di]
- RaH::
-
Mass transfer Rayleigh number based on enclosure height [g(ρbulk-ρc)H3/ρν Di]
- Rax::
-
Local mass transfer Rayleigh number [g(ρbulk-ρc) x3/ρν Di]
- Sc::
-
Schmidt number (ν/Di)
- Sh::
-
Sherwood number (hL/Di)
- Shx::
-
Local Sherwood number (hx/Di)
- ti::
-
Transference number
- W::
-
Width of cathode plate (m)
- x::
-
Position from leading edge of cathode surface (m)
- δ::
-
Boundary layer thickness (m)
- λr::
-
Width between adjacent rolls (m)
- ν::
-
Kinematic viscosity (m2/s)
- θ::
-
Angle of enclosure inclination from horizontal (degrees)
- θ*::
-
Transition angle from longitudinal rolls to unicellular flow (degrees)
- ρ::
-
Density (kg/m3)
References
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Goldstein, R.J., Chiang, H.D., Srinivasan, V. et al. Local mass transfer measurements in an inclined enclosure at high Rayleigh number. Heat Mass Transfer 41, 991–998 (2005). https://doi.org/10.1007/s00231-005-0630-0
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DOI: https://doi.org/10.1007/s00231-005-0630-0