Abstract
Ultrashort laser pulses are used to ablate a thin molybdenum layer from glass by irradiating the metal film through the transparent substrate. The trajectories of ablated molybdenum fragments are recorded using a shadowgraphic setup with a time resolution in the nanosecond range. In addition, the shape of collected molybdenum fragments is examined as a function of applied fluence. It is confirmed that in a fluence regime close to the ablation threshold one single disc is ablated as a whole and its velocity is determined in the order of 50 ms−1. In a second fluence regime, partial melting at the center of the disc is found and small melt droplets are recorded on their flight. Mo fragments ablated in this regime feature a ring-like structure with a brittle fracture at the outer and a molten appearance at the inner edge.
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B. Chichkov, C. Momma, S. Nolte, F. Von Alvensleben, A. Tünnermann, Appl. Phys. A 63(2), 109 (1996). doi:10.1007/s003390050359
S. Nolte, C. Momma, H. Jacobs, A. Tünnermann, B. Chichkov, B. Wellegehausen, H. Welling, J. Opt. Soc. Am. B 14(10), 2716 (1997). doi:10.1364/JOSAB.14.002716
D. Breitling, A. Ruf, F. Dausinger, Proc. SPIE 5339(1), 49 (2004). doi:10.1117/12.541434
R. Knappe, T. Herrmann, B. Heinrich, A. Nebel, in Proc. 3rd Int. WLT-Conf. on Lasers in Manuf. (2005), pp. 723–728
F. Röser, T. Eidam, J. Rothhardt, O. Schmidt, D. Schimpf, J. Limpert, A. Tünnermann, Opt. Lett. 32(24), 3495 (2007). doi:10.1364/OL.32.003495
J. Kleinbauer, D. Eckert, S. Weiler, D.H. Sutter, Proc. SPIE 6871(1), 68711B (2008). doi:10.1117/12.760981
P. Russbueldt, T. Mans, G. Rotarius, J. Weitenberg, H.D. Hoffmann, R. Poprawe, Opt. Express 17(15), 12230 (2009). doi:10.1364/OE.17.012230
J. König, T. Bauer, Proc. SPIE 7925(1), 792510 (2011). doi:10.1117/12.878593
D. Ruthe, K. Zimmer, T. Höche, Appl. Surf. Sci. 247(1–4), 447 (2005). doi:10.1016/j.apsusc.2005.01.048
J. Hermann, M. Benfarah, S. Bruneau, E. Axente, G. Coustillier, T. Itina, J.F. Guillemoles, P. Alloncle, J. Phys. D, Appl. Phys. 39(3) (2006). doi:10.1088/0022-3727/39/3/005
S. Zoppel, H. Huber, G. Reider, Appl. Phys. A 89(1), 161 (2007). doi:10.1007/s00339-007-4158-7
H.P. Huber, F. Herrnberger, S. Kery, S. Zoppel, Proc. SPIE 6881(1), 688117 (2008). doi:10.1117/12.767821
T. Dalibor, S. Jost, H. Vogt, A. Heiß, S. Visbeck, T. Happ, J. Palm, A. Avellán, T. Niesen, F. Karg, in Proc. 26th EUPVSEC (2011), pp. 2407–2411. doi:10.4229/26thEUPVSEC2011-3CO.2.1
A.B. Bullock, P.R. Bolton, J. Appl. Phys. 85(1), 460 (1999). doi:10.1063/1.369393
H.P. Huber, M. Englmaier, C. Hellwig, A. Heiss, T. Kuznicki, M. Kemnitzer, H. Vogt, R. Brenning, J. Palm, Proc. SPIE 7203(1), 72030R (2009). doi:10.1117/12.812332
G. Heise, M. Englmaier, C. Hellwig, T. Kuznicki, S. Sarrach, H.P. Huber, Appl. Phys. A 102, 173 (2011). doi:10.1007/s00339-010-5993-5
F.J. Mayer, G.E. Busch, J. Appl. Phys. 57(3), 827 (1985). doi:10.1063/1.334733
A.B. Bullock, P.R. Bolton, F.J. Mayer, J. Appl. Phys. 82(4), 1828 (1997). doi:10.1063/1.366289
V. Schultze, M. Wagner, Appl. Phys. A 53, 241 (1991). doi:10.1007/BF00324259
Y. Nakata, T. Okada, Appl. Phys. A 69, S275 (1999). doi:10.1007/s003390051399
R. Fardel, M. Nagel, F. Nüesch, T. Lippert, A. Wokaun, Appl. Surf. Sci. 255(10), 5430 (2009). doi:10.1016/j.apsusc.2008.07.187
K.S. Kaur, R. Fardel, T.C. May-Smith, M. Nagel, D.P. Banks, C. Grivas, T. Lippert, R.W. Eason, J. Appl. Phys. 105(11), 113119 (2009). doi:10.1063/1.3132822
D.G. Papazoglou, A. Karaiskou, I. Zergioti, C. Fotakis, Appl. Phys. Lett. 81(9), 1594 (2002). doi:10.1063/1.1497191
A. Kuznetsov, C. Unger, J. Koch, B. Chichkov, Appl. Phys. A 106, 479 (2012). doi:10.1007/s00339-011-6747-8
M. Domke, G. Heise, I. Richter, S. Sarrach, H.P. Huber, Phys. Procedia 12(Part 2), 399 (2011). doi:10.1016/j.phpro.2011.03.149
M. Domke, S. Rapp, M. Schmidt, H.P. Huber, Opt. Express 20(9), 10330 (2012). doi:10.1364/OE.20.010330
A. Michalowski, D. Walter, P. Berger, F. Dausinger, in Proc. 4th Int. WLT-Conf. on Lasers in Manuf. (2007), pp. 563–567
D.W. Lynch, W.R. Hunter, Handbook of Optical Constants of Solids (Academic Press, San Diego, 1985), pp. 303–313, Chap. VI
J.M. Liu, Opt. Lett. 7(5), 196 (1982)
Acknowledgements
We acknowledge financial support by the German Federal Ministry of Education and Research (BMBF) under contract Nos. 13N11783 and 13N11788 (“Tailored for next PV, T4nPV”).
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Bartl, D., Michalowski, A., Hafner, M. et al. Time-resolved study of back side ablated molybdenum thin films by ultrashort laser pulses. Appl. Phys. A 110, 227–233 (2013). https://doi.org/10.1007/s00339-012-7118-9
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DOI: https://doi.org/10.1007/s00339-012-7118-9