Skip to main content
Log in

Piezoelectric BNT-BT0.11 thin films processed by sol–gel technique

  • Published:
Journal of Materials Science Aims and scope Submit manuscript

Abstract

0.89(Na0.5Bi0.5)TiO3–0.11BaTiO3, (BNT-BT0.11) thin film was fabricated by sol–gel/spin coating process, on platinized silicon wafer. Perovskite structure with random orientation of crystallites has been obtained at 700 °C. Piezoelectric activity of BNT-BT0.11 thin film was detected using piezoresponse force microscopy (PFM). Effective piezoelectric coefficient d33eff of such film, recorded at 5 V applied dc voltage, was ~29 pm/V, which is similar to other BNT-BTx thin films. The complex refractive index and dielectric function of BNT-BT0.11 thin films were also investigated. The high leakage current density significantly influences the dielectric, ferroelectric, and piezoelectric properties of the BNT-BT0.11 films.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9
Fig. 10
Fig. 11
Fig. 12

Similar content being viewed by others

References

  1. Hiruma Y, Watanabe Y, Nagata H, Takenaka T (2007) Key Eng Mater 350:93

    Article  CAS  Google Scholar 

  2. Zvirgzds JA, Kapostis PP, Zvirgzde JV (1982) Ferroelectrics 40:75

    Article  CAS  Google Scholar 

  3. Trujillo S, Kreisel J, Jiang Q, Smith JH, Thomas PA, Bouvier P, Weiss F (2005) J Phys 17:6587

    CAS  Google Scholar 

  4. Chiang YM, Farrey GW, Soukhojak AN (1998) Appl Phys Lett 73:3683

    Article  CAS  Google Scholar 

  5. Takenaka T, Maruyama K, Sakata K (1991) Jpn J Appl Phys 30:2236

    Article  CAS  Google Scholar 

  6. Chu BJ, Chen DR, Li GR, Yin QR (2002) J Eur Ceram Soc 22:2115

    Article  CAS  Google Scholar 

  7. Chen M, Xu Q, Kim BH, Ahn BK, Ko JH, Kang WJ, Nam OJ (2008) J Eur Ceram Soc 28:843

    Article  Google Scholar 

  8. Rout D, Moon KS, Rao VS, Kang SJL (2009) J Ceram Soc Jpn 117:797

    Article  CAS  Google Scholar 

  9. Yilmaz H, Messing GL, Trolier-McKinstry S (2003) J Electroceram 11:207

    Article  CAS  Google Scholar 

  10. Yilmaz H, Trolier-McKinstry S, Messing GL (2003) J Electroceram 11:217

    Article  CAS  Google Scholar 

  11. Alonso-Sanjose D, Jimenez R, Bretos I, Calzada ML (2009) J Am Ceram Soc 92:2218

    Article  CAS  Google Scholar 

  12. Cernea M, Andronescu E, Radu R, Fochi F, Galassi C (2010) J Alloy Compd 490:690

    Article  CAS  Google Scholar 

  13. Ge W, Liu H, Zhao X, Pan X, He T, Lin D, Xu H, Luo H (2008) J Alloy Compd 456:503

    Article  CAS  Google Scholar 

  14. Zhang ST, Kounga AB, Aulbach E, Deng Y (2008) J Am Ceram Soc 91:3950

    Article  CAS  Google Scholar 

  15. Cheng HW, Zhang XJ, Zhang ST, Feng Y, Chen YF, Liu ZG, Liu GX (2004) Appl Phys Lett 85:2319

    Article  CAS  Google Scholar 

  16. Dinescu M, Craciun F, Scarisoreanu N, Verardi P, Moldovan A, Purice A, Sanson A, Galassi C (2005) J Phys IV France 128:77

    Article  CAS  Google Scholar 

  17. Scarisoreanu N, Craciun F, Ion V, Birjega S, Dinescu M (2007) Appl Surf Sci 254:1992

    Article  Google Scholar 

  18. Zhang DZ, Zheng XJ, Feng X, Zhang T, Sun J, Dai SH, Gong LJ, Gong YQ, He L, Zhu Z, Huang J, Xu X (2010) J Alloy Compd 504:129

    Article  CAS  Google Scholar 

  19. Brinker J, Scherer GW (1990) Sol-gel science: the physics and chemistry of sol-gel processing. Academic Press Inc, Boston

    Google Scholar 

  20. Ryu SO (1999) Synthesis and characterization of ferroelectric (1 − x)SrBi2Ta2O9xBi3TaTiO9 thin films for non-volatile memory applications. https://doi.org/scholar.lib.vt.edu/theses/available/etd-050699-154541/unrestricted/Chapter5.pdf

  21. Chang DA, Choh YH, Hsieh WF, Lin P, Tseng TY (1993) J Mater Sci 28:6691. doi:https://doi.org/10.1007/BF00356416

    Article  CAS  Google Scholar 

  22. Fujiwara H (2007) Spectroscopic ellipsometry: principles and applications. Wiley, West Sussex

    Book  Google Scholar 

  23. Bass M (ed) (2009) Handbook of optics, 3rd edn, vol 4: optical properties of materials, nonlinear optics, quantum optics. McGraw-Hill Comp, Inc., New York

    Google Scholar 

  24. Ferlauto AS, Ferreira GM, Pearce JM, Wronski CR, Collins RW, Deng X, Ganguly G (2002) J Appl Phys 92:2424

    Article  CAS  Google Scholar 

  25. Stan GE, Pasuk I, Galca AC, Dinescu A (2010) Dig J Nanomater Biostruct 5:1041

    Google Scholar 

  26. Ma C, Tan X (2010) Solid State Commun 150:497

    Google Scholar 

  27. Zhou ZH, Xue JM, Li WZ, Wang J, Zhu H, Miao JM (2004) Appl Phys Lett 85:804

    Article  CAS  Google Scholar 

  28. Takenaka T, Sakata K (1989) Ferroelectrics 95:153

    Article  CAS  Google Scholar 

Download references

Acknowledgement

We thank the Romanian National Program PNCDI II, Contract No. 72-153/2008, and the Romanian National Authority for Scientific Research (PN09-450101, Contract No. 45N/1.03.2009) for the financial support.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Marin Cernea.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Cernea, M., Galca, A.C., Cioangher, M.C. et al. Piezoelectric BNT-BT0.11 thin films processed by sol–gel technique. J Mater Sci 46, 5621–5627 (2011). https://doi.org/10.1007/s10853-011-5512-x

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10853-011-5512-x

Keywords

Navigation