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Pulsed Laser Deposition Films Based on CdSe-Doped Zinc Aluminophosphate Glass

  • Advanced Coating and Thin Film Materials for Energy, Aerospace and Biological Applications
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Abstract

A composite material with applications in optoelectronics has been investigated. Pulsed laser deposition CdSe-doped glass film was prepared by the combinatorial deposition from two targets, namely pure CdSe and glass belonging to the 20Li2O-10Al2O3-7BaO-2La2O3-2ZnO-59P2O5 system. Exciton peaks in the Vis domain, related to electron–hole pairs transitions from the valence band to the conduction band, were revealed in the optical absorption spectra of the CdSe-doped film. CdSe quantum dots (QDs) band gap energy depends on the CdSe quantum confinement effect. CdSe-doped film photoluminescence exhibits peaks in the red domain assigned to CdSe transitions from the excited state to the ground state. The size of CdSe nanoclusters, determined from x-ray diffraction is correlated with scanning electron microscopy–energy dispersive x-ray spectroscopy and atomic force microscopy results. Vibration modes specific both to CdSe QDs and to the vitreous network have been evidenced by Fourier transform infrared and Raman spectroscopy.

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Acknowledgements

The authors acknowledge the funding from the Ministry of Research and Innovation through Program I- Development of the National Research and Development System, Subprogram 1.2 - Institutional Performance-Projects for Excellence Financing in RDI, Contract No.19PFE/17.10.2018, and contracts 47PCCDI/2018, 42PCCDI/2018, PN 16N/2019, PN 18N/2019, and PN 21N/2019.

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  1. National Institute of R & D for Optoelectronics - INOE 2000, 077125, Magurele, Ilfov, Romania

    Mihail Elisa, Stefan-Marian Iordache, Ana-Maria Iordache & Madalin Ion Rusu

  2. National Institute for Laser, Plasma and Radiation Physics, 077125, Magurele, Ilfov, Romania

    Gabriel Socol & Mihaela Filipescu

  3. National Institute of Materials Physics, 077125, Magurele, Ilfov, Romania

    Cristina Bartha & Monica Enculescu

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  1. Mihail Elisa
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Elisa, M., Iordache, SM., Iordache, AM. et al. Pulsed Laser Deposition Films Based on CdSe-Doped Zinc Aluminophosphate Glass. JOM 73, 495–503 (2021). https://doi.org/10.1007/s11837-020-04150-3

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