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Dielectric properties and electromagnetic simulation of molybdenum disulfide and ferric oxide-modified Ti3C2TX MXene hetero-structure for potential microwave absorption

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Abstract

As newly emerged 2D materials, Ti3C2TX MXene have exhibited great potential to be used as high-performance microwave absorption materials (MAs). In this study, multilayer accordion-like Ti3C2TX MXene coated by molybdenum disulfide (Ti3C2TX@MoS2) and ferric oxide (Ti3C2TX@Fe2O3) were fabricated through hydrothermal method. The dielectric properties of the paraffin wax consisting of 50 wt% Ti3C2TX, Ti3C2TX@MoS2, and Ti3C2TX@Fe2O3 were evaluated in 2–18 GHz, respectively. It is found that Ti3C2TX@MoS2 and Ti3C2TX@Fe2O3 displayed enhanced impedance matching than pure Ti3C2TX. The as-fabricated composites showed great potential for microwave absorption, for sample Ti3C2TX@MoS2 (mass ratio 1:1), which has the largest reflection loss (RL) value of − 60.2 dB at 16.6 GHz. The Ti3C2TX@Fe2O3 achieved optimal RL of − 18.6 dB at 17.4 GHz with thickness of 1.97 mm, and the effective absorption bandwidth (EAB) achieved 4.3 GHz (13.4–17.7 GHz) corresponding to thickness of 2.25 mm. The attenuation mechanisms were clarified by high-frequency structure simulator (HFSS). The interface polarization and multi-scattering make the dominant contributions for the improved microwave absorption.

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Acknowledgements

The author would like to thank Xiaoli Fan from Shiyanjia Lab (www.shiyanjia.com) for the XRD analysis.

Funding

The authors acknowledge the financial support of Taif University Researchers Supporting Project number (TURSP-2020/05), Taif University, Taif, Saudi Arabia. The authors also acknowledge the support from the Natural Science Foundation of Shandong Province (ZR2021QE164), the National Natural Science Foundation of China (No. 51872173), the Taishan Scholar Foundation of Shandong Province (No. tsqn201812068), the Youth Innovation Technology Project of Higher School in Shandong Province (No. 2019KJA013), and Science and Technology Special Project of Qingdao City (No. 20–3-4–3-nsh).

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Authors and Affiliations

  1. School of Material Science and Engineering, Shandong University of Science and Technology, Qingdao, 266590, People’s Republic of China

    Nannan Wu, Beibei Zhao, Xiaoyue Chen & Jian Tian

  2. School of Environmental and Material Engineering, Yantai University, No. 30 Qingquan Road, Yantai, 264005, Shandong, China

    Chuanxin Hou

  3. Department of Chemistry, College of Science, Taif University, P.O. Box 11099, Taif, 21944, Saudi Arabia

    A. Alhadhrami, Gaber A. M. Mersal & Mohamed M. Ibrahim

  4. College of Materials Science and Engineering, Taiyuan University of Science and Technology, Taiyuan, 030024, China

    Mina Huang

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Wu, N., Zhao, B., Chen, X. et al. Dielectric properties and electromagnetic simulation of molybdenum disulfide and ferric oxide-modified Ti3C2TX MXene hetero-structure for potential microwave absorption. Adv Compos Hybrid Mater 5, 1548–1556 (2022). https://doi.org/10.1007/s42114-022-00490-7

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