Abstract
We present the first single-crystal study of Fe and Ni doped U(Co1-x T x )Al compounds in comparison to the parent compound, the itinerant 5f-electron metamagnet UCoAl. Magnetization and specific-heat data measured in the temperature range of (1.8-300) K and in fields up to 10 T are analyzed and discussed. Both compounds exhibit a strong uniaxial anisotropy with the dominating magnetic response along the c-axis of the hexagonal ZrNiAl-type structure. Ni substitution yields an increase of the critical field for metamagnetism; UCo0.95Fe0.05Al is ferromagnetic below 30 K. Temperature evolution of the entropy change between 0 and 10 T points to involvement of magnetic correlations or spin fluctuations in the paramagnetic compounds UCoAl and UCo0.95Ni0.05Al.
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Andreev, A., Janoušová, B., Sechovský, V. et al. Magnetization and Specific Heat of UCo0.95T0.05Al (T = Fe, Ni) Single Crystals. Czechoslovak Journal of Physics 52, 275–278 (2002). https://doi.org/10.1023/A:1014448519010
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DOI: https://doi.org/10.1023/A:1014448519010