Abstract
Manipulation of light is in strong demand in information technologies. Among the wide range of linear and nonlinear optical devices that have been used, growing attention has been paid to photonic crystals that possess a periodic modulation of dielectric function1,2. Among many photonic bandgap (PBG) structures, liquid crystals with periodic structures are very attractive as self-assembled photonic crystals3, leading to optical devices such as dye lasers4,5. Here we report a new hetero-PBG structure consisting of an anisotropic nematic layer sandwiched between two cholesteric liquid-crystal layers with different helical pitches. We optically visualized the dispersion relation of this structure, displaying the optical diode performance: that is, the non-reciprocal transmission of circular polarized light at the photonic-bandgap regions. Transmittance spectra with circularly polarized light also reveal the diode performance, which is well simulated in calculations that include an electro-tunable diode effect. Lasing action was also confirmed to show the diode effect with a particular directionality.
This is a preview of subscription content, access via your institution
Access options
Subscribe to this journal
Receive 12 print issues and online access
$259.00 per year
only $21.58 per issue
Buy this article
- Purchase on Springer Link
- Instant access to full article PDF
Prices may be subject to local taxes which are calculated during checkout
Similar content being viewed by others
References
Yablonovitch, E. Inhibited spontaneous emission in solid-state physics and electronics. Phys. Rev. Lett. 58, 2059–2062 (1987).
Joannopoulos, J. D., Villeneuve, P. R. & Fan, S. Photonic crystals: putting a new twist on light. Nature 386, 143–149 (1997).
De Gennes, P. G. & Prost, J. The Physics of Liquid Crystals 2nd edn, Ch. 6 (Clarendon, Oxford, 1993).
Kopp, V. I., Fan, B., Vithana, H. K. M. & Genack, A. Z. Low-threshold lasing at the edge of a photonic stop band in cholesteric liquid crystals. Opt. Lett. 23, 1707–1709 (1998).
Song, M. H. et al. Effect of phase retardation on defect mode lasing in polymeric cholesteric liquid crystals. Adv. Mater. 16, 779–783 (2004).
Bouligand, Y. Sur l'existence de 'Pseudomorphoses cholesteriques' chez divers organisms vivants. J. Phys. (Paris) C 4, 30, 90–103 (1969).
Caveney, S. Cuticle reflectivity and optical activity in scarab beetles: the role of uric acid. Proc. R. Soc. Ser. B 178, 205–225 (1971).
Scalora, M., Dowling, J. P. Bowden, C. M. & Bloemer, M. J. The photonic band edge optical diode. J. Appl. Phys. 76, 2023–2026 (1994).
Mingaleev, S. F. & Kivshar, Y. S. Nonlinear transmission and light localization in photonic-crystal waveguides. J. Opt. Soc. Am. B 19, 2241–2249 (2002).
Mujumdar, S. & Ramachandran, H. Use of a graded gain random amplifier as an optical diode. Opt. Lett. 26, 929–931 (2001).
Gevorgyan, A. H. Optical diode based on a highly anisotropic layer of a helical periodic medium subjected to a magnetic field. Tech. Phys. 47, 1008–1013 (2002).
Gevorgyan, A. H. Nonreciprocal waves in absorbing multilayer systems. Tech. Phys. Lett. 29, 60–68 (2003).
Tocci, M. D., Bloemer, M. J., Scalora, M., Dowling, J. P. & Bowden, C. M. Thin-film nonlinear optical diode. Appl. Phys. Lett. 66, 2324–2326 (1995).
Berreman, D. W. Optics in stratified and anisotropic media: 4 × 4-matrix formation. J. Opt. Soc. Am. 62, 502–510 (1972).
Song, M. H. et al. Polarization characteristic of phase retardation defect mode lasing in polymeric cholesteric cholesteric liquid crystals. Sci. Technol. Adv. Mater. 5, 437–441 (2004).
Long, T. M. & Swager, T. M. Using internal free volume to increase chromophore alignment. J. Am. Chem. Soc. 124, 3826–3827 (2002).
Acknowledgements
The laser dye used in this study was supplied from T. M. Swager (MIT). The work is supported by JSPS through the TIT-KAIST core university corroboration program, KOSEF through ABRL program at Ewha Womans University, 21st COE program of Materials Science in Tokyo Tech and a Grant-in-Aid for Exploratory Research (16656023) by the Ministry of Education, Science, Sports and Culture of Japan.
Author information
Authors and Affiliations
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing financial interests.
Rights and permissions
About this article
Cite this article
Hwang, J., Song, M., Park, B. et al. Electro-tunable optical diode based on photonic bandgap liquid-crystal heterojunctions. Nature Mater 4, 383–387 (2005). https://doi.org/10.1038/nmat1377
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1038/nmat1377
This article is cited by
-
Uniformly aligned flexible magnetic films from bacterial nanocelluloses for fast actuating optical materials
Nature Communications (2022)
-
Analyzing two-dimensional tunable photonic crystal waveguides for communication band optical filter applications
Journal of Optics (2021)
-
Acoustic radiation pressure for nonreciprocal transmission and switch effects
Nature Communications (2019)
-
Broadband high contrast ratio optical diodes based on polarization conversion
Applied Physics B (2017)
-
On-Chip Optical Nonreciprocity Using an Active Microcavity
Scientific Reports (2016)