Issue 80, 2016
From the journal:

Chemical Communications

Hierarchical silicalite-1 octahedra comprising highly-branched orthogonally-stacked nanoplates as efficient catalysts for vapor-phase Beckmann rearrangement†

Albert Chang,a   Hsu-Ming Hsiao,a   Tsai-Hsiu Chen,a   Ming-Wen Chub  and  Chia-Min Yang*ac  

* Corresponding authors

a Department of Chemistry, National Tsing Hua University, Hsinchu 30013, Taiwan
E-mail: cmyang@mx.nthu.edu.tw

b Center for Condensed Matter Sciences, National Taiwan University, Taipei 10617, Taiwan

c Frontier Research Center on Fundamental and Applied Sciences of Matters, National Tsing Hua University, Hsinchu 30013, Taiwan

Abstract

A triblock structure-directing agent was designed to synthesize hierarchical silicalite-1 octahedra comprising highly-branched, orthogonally-stacked and self-pillared nanoplates that exhibited excellent and stable activity for the vapor-phase Beckmann rearrangement of cyclic oximes and high lactam selectivity.

Graphical abstract: Hierarchical silicalite-1 octahedra comprising highly-branched orthogonally-stacked nanoplates as efficient catalysts for vapor-phase Beckmann rearrangement

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Article information

DOI
https://doi.org/10.1039/C6CC05992A
Article type
Communication
Submitted
21 Jul 2016
Accepted
08 Sep 2016
First published
08 Sep 2016

Chem. Commun., 2016,52, 11939-11942

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Hierarchical silicalite-1 octahedra comprising highly-branched orthogonally-stacked nanoplates as efficient catalysts for vapor-phase Beckmann rearrangement

A. Chang, H. Hsiao, T. Chen, M. Chu and C. Yang, Chem. Commun., 2016, 52, 11939 DOI: 10.1039/C6CC05992A

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