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Reading diffraction images in strong field ionization of diatomic molecules

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Published 27 May 2004 2004 IOP Publishing Ltd
, , Citation Michael Spanner et al 2004 J. Phys. B: At. Mol. Opt. Phys. 37 L243 DOI 10.1088/0953-4075/37/12/L02

0953-4075/37/12/L243

Abstract

We present a theoretical analysis of how intense, few-cycle infrared laser pulses can be used to image the structure of small molecules with nearly 1 fs temporal and sub-Å spatial resolution. We identify and analyse several physical mechanisms responsible for the distortions of the diffraction image and describe a recipe for recovering an un-distorted image from angle and energy-resolved electron spectra. We also identify holographic patterns in the photoelectron spectra and discuss the requirements to enhancing the hologram resolution for imaging the scattering potential.

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10.1088/0953-4075/37/12/L02