Directional dark-field implicit x-ray speckle tracking using an anisotropic-diffusion Fokker-Planck equation

Konstantin M. Pavlov, David M. Paganin, Kaye S. Morgan, Heyang (Thomas) Li, Sebastien Berujon, Laurène Quénot, and Emmanuel Brun
Phys. Rev. A 104, 053505 – Published 2 November 2021

Abstract

When a macroscopic-sized noncrystalline sample is illuminated using coherent x-ray radiation, a bifurcation of photon energy flow may occur. The coarse-grained complex refractive index of the sample may be considered to attenuate and refract the incident coherent beam, leading to a coherent component of the transmitted beam. Spatially unresolved sample microstructure, associated with the fine-grained components of the complex refractive index, introduces a diffuse component to the transmitted beam. This diffuse photon-scattering channel may be viewed in terms of position-dependent fans of ultrasmall-angle x-ray scatter. These position-dependent fans, at the exit surface of the object, may under certain circumstances be approximated as having a locally elliptical shape. By using an anisotropic-diffusion Fokker-Planck approach to model this bifurcated x-ray energy flow, we show how all three components (attenuation, refraction, and locally elliptical diffuse scatter) may be recovered. This is done via x-ray speckle tracking, in which the sample is illuminated with spatially random x-ray fields generated by coherent illumination of a spatially random membrane. The theory is developed and then successfully applied to experimental x-ray data.

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  • Received 26 May 2021
  • Accepted 23 September 2021

DOI:https://doi.org/10.1103/PhysRevA.104.053505

©2021 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

Konstantin M. Pavlov*

  • School of Physical and Chemical Sciences, University of Canterbury, Christchurch 8140, New Zealand; School of Physics and Astronomy, Monash University, Melbourne, Victoria 3800, Australia; and School of Science and Technology, University of New England, Armidale, New South Wales 2351, Australia

David M. Paganin and Kaye S. Morgan

  • School of Physics and Astronomy, Monash University, Melbourne, Victoria 3800, Australia

Heyang (Thomas) Li

  • School of Mathematics and Statistics, University of Canterbury, Christchurch 8140, New Zealand

Sebastien Berujon

  • Instituto COPPEAD de Administração, Universidade Federal do Rio de Janeiro, Rio de Janeiro, Rio de Janeiro 21941-918, Brazil

Laurène Quénot and Emmanuel Brun

  • Université Grenoble Alpes, Inserm UA7, 38000 Grenoble, France

  • *konstantin.pavlov@canterbury.ac.nz

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Issue

Vol. 104, Iss. 5 — November 2021

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