Abstract
Two-photon absorption cross sections for transitions from the OP) ground electronic state to the 3p P, 4p P, and the autoionizing (D)3p’ and (P)3p’’ states have been calculated by explicit evaluation of the perturbation-theory summation using matrix elements calculated from configuration-interaction wave functions and sum rules to correct for truncation. The role of different contributions in the summation has been analyzed. For the 3p P state, a cross section of (J’←J) of (1.319±0.2)× has been obtained, which is in excellent agreement with the experimental value for the quantity (J’←2) =(2.66±0.80)× , given in the companion paper, if the photon statistical factor, , is evaluated in the chaotic field limit (=2).
- Received 3 February 1986
DOI:https://doi.org/10.1103/PhysRevA.34.199
©1986 American Physical Society