Theory of Saturated-Absorption Line Shapes

Serge Haroche and Francis Hartmann
Phys. Rev. A 6, 1280 – Published 1 October 1972
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Abstract

A general theory of the saturated-absorption phenomenon in a two-level atomic system is developed, in which the phase relationships between the oscillating atomic dipoles as well as the population differences between energy levels are taken into account. The absorbing gaseous medium considered in this theory is subjected to irradiation by a quasi-running-wave composed of a strong pump field and a weak probe field propagating in opposite directions. Some new interesting results, not predicted by the so-called hole-burning or rate-equation model, are obtained. In particular, the probe-field-transmission peak line shape is found to be markedly different from what is expected according to the rate equations. For finite Doppler widths and a strong saturating pump field, absorption of the probe field can even change sign, and amplification of this field can actually occur. All these features are explained by a close inspection of the evolution of each atomic ensemble of given velocity. Detailed comparison with similar phenomena already observed in rf experiments is presented and permits us to clarify the new predicted effects.

  • Received 30 March 1972

DOI:https://doi.org/10.1103/PhysRevA.6.1280

©1972 American Physical Society

Authors & Affiliations

Serge Haroche*

  • Laboratoire de l'Horloge Atomique du Centre National de la Recherche Scientifique, 91 Orsay, France and Laboratoire de Spectroscopie Hertzienne de l'Ecole Normale Superieure, 24 rue Lhomond, Paris 5e, France

Francis Hartmann

  • Laboratoire de l'Horloge Atomique du Centre National de la Recherche Scientifique, 91 Orsay, France

  • *Permanent address.

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Issue

Vol. 6, Iss. 4 — October 1972

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