Quantum-mechanical-model calculations of radiative properties of a molecular crystal. I. Polaritons and abnormal decays of excitons in one- and two-dimensional systems

Michel Orrit, Claude Aslangul, and Philémon Kottis
Phys. Rev. B 25, 7263 – Published 15 June 1982
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Abstract

An analysis of the interaction of an electronic collective excitation, of dimensions 1 and 2, with the radiation field is presented. The use of translation symmetry in infinite lattices allows us to reduce the interaction problem to a coupling of a discrete matter state to an effective continuum of photons presenting a low-energy edge. The resulting states (radiatively unstable excitons, polaritons) are investigated as a function of the electronic excitation energy relative to the edge of the continuum, with emphasis on the spectral properties and the dynamical regimes in the intermediate region, when the energy of the electronic excitation sweeps the edge of the continuum. Contact with the three-dimensional polariton is made while application to radiative dynamics in layered crystals is suggested.

  • Received 31 January 1980

DOI:https://doi.org/10.1103/PhysRevB.25.7263

©1982 American Physical Society

Authors & Affiliations

Michel Orrit, Claude Aslangul*,†, and Philémon Kottis

  • Centre de Physique Moléculaire, Optique et Hertzienne, University of Bordeaux I, 33405 Talence, France
  • Centre de Mecanique Ondulatoire Appliquée, 23, Rue du Maroc, 75019, Paris, France

  • *Present address: Groupe de Physique Solides des l'Ecole Normal Superieure, Universite de Paris VII, 75221 Paris, France.
  • Laboratory associated with CNRS (LA 283).

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Vol. 25, Iss. 12 — 15 June 1982

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