Abstract
The magnetic susceptibility and specific heat of the diluted magnetic semiconductor Se have been measured in the temperature range 10 mK<T<40 K for 0.01≤x≤0.53. A paramagnetic–spin-glass transition was observed in the whole concentration range. The concentration dependence of the freezing temperature was found to be compatible with a radial dependence of the exchange interaction between manganese ions of the type J(R)∼. Based on this observation, we calculated thermodynamic properties with the extended nearest-neighbor pair approximation. It appears that this approximation provides a good simultaneous description of the specific heat and high-field magnetization and reproduces Curie-Weiss temperature for parameters /=-13 K (nearest-neighbor interaction) and (R)/=-7/ K (distant-neighbor interaction). A comparison is made with other dilute magnetic semiconductors, and the possible origin of the exchange mechanism is then discussed.
- Received 26 March 1987
DOI:https://doi.org/10.1103/PhysRevB.36.7013
©1987 American Physical Society