Spontaneous emission spectra and quantum light-matter interactions from a strongly coupled quantum dot metal-nanoparticle system

C. Van Vlack, Philip Trøst Kristensen, and S. Hughes
Phys. Rev. B 85, 075303 – Published 3 February 2012

Abstract

We investigate the quantum optical properties of a quantum-dot dipole emitter coupled to a finite-size metal nanoparticle using a photon Green-function technique that rigorously quantizes the electromagnetic fields. We first obtain pronounced Purcell factors and photonic Lamb shifts for both a 7- and 20-nm-radius metal nanoparticle, without adopting a dipole approximation. We then consider a quantum-dot photon emitter positioned sufficiently near the metal nanoparticle so that the strong-coupling regime is possible. Accounting for nondipole interactions, quenching, and photon transport from the dot to the detector, we demonstrate that the strong-coupling regime should be observable in the far-field spontaneous emission spectrum, even at room temperature. The vacuum-induced emission spectra show that the usual vacuum Rabi doublet becomes a rich spectral triplet or quartet with two of the four peaks anticrossing, which survives in spite of significant nonradiative decays. We discuss the emitted light spectrum and the effects of quenching for two different dipole polarizations.

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  • Received 22 December 2011

DOI:https://doi.org/10.1103/PhysRevB.85.075303

©2012 American Physical Society

Authors & Affiliations

C. Van Vlack1,*, Philip Trøst Kristensen2, and S. Hughes1

  • 1Queen's University, Department of Physics, Kingston Ontario, Canada K7L 3N6
  • 2DTU Fotonik, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark

  • *cvanvlack@physics.queensu.ca

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Vol. 85, Iss. 7 — 15 February 2012

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