Aging dynamics in a colloidal glass

Bérengère Abou, Daniel Bonn, and Jacques Meunier
Phys. Rev. E 64, 021510 – Published 24 July 2001
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Abstract

The aging dynamics of colloidal suspensions of Laponite, a synthetic clay, is investigated using dynamic light scattering (DLS) and viscometry after a quench into the glassy phase. DLS allows to follow the diffusion of Laponite particles and reveals that there are two modes of relaxation. The fast mode corresponds to a rapid diffusion of particles within “cages” formed by the neighboring particles. The slow mode corresponds to escape from the cages: its average relaxation time increases exponentially fast with the age of the glass. In addition, the slow mode has a broad distribution of relaxation times, its distribution becoming larger as the system ages. Measuring the concomitant increase of viscosity as the system ages, we can relate the slowing down of the particle dynamics to the viscosity.

  • Received 26 January 2001

DOI:https://doi.org/10.1103/PhysRevE.64.021510

©2001 American Physical Society

Authors & Affiliations

Bérengère Abou, Daniel Bonn, and Jacques Meunier

  • Laboratoire de Physique Statistique, Ecole Normale Supérieure 24, rue Lhomond, 75231 Paris, France

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Issue

Vol. 64, Iss. 2 — August 2001

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