Optical gratings formed in thin smectic films frustrated on a single crystalline substrate

Jean-Philippe Michel, Emmanuelle Lacaze, Michel Alba, Marc de Boissieu, Marc Gailhanou, and Michel Goldmann
Phys. Rev. E 70, 011709 – Published 30 July 2004

Abstract

Through the combination of three different, complementary techniques (optical microscopy, x-ray diffraction and atomic force microscopy), we reveal the deformations inside thin smectic films frustrated between two interfaces imposing antagonistic anchorings. We study the model system, 4-n-octyl-4-cyanobiphenyl (8CB) between MoS2 and air, which is characterized by the competition between homeotropic anchoring at air and planar unidirectional anchoring on the substrate, with thicknesses varying around 0.3μm. Optical microscopy and x-ray diffraction demonstrate the continuous topology of smectic layers between the interfaces, which are stacked into periodic flattened hemicylinders. These latter are one-dimensional (1D) focal conic domains which form an optical grating in the smectic film, of a period ranging from 1 to 2.5μm. The interpretation of our results through an energetic model, associated with the atomic force microscopy (AFM) measurements, shows the presence below a critical thickness of a new type of curvature wall between neighboring hemicylinders.

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  • Received 4 December 2003

DOI:https://doi.org/10.1103/PhysRevE.70.011709

©2004 American Physical Society

Authors & Affiliations

Jean-Philippe Michel and Emmanuelle Lacaze*

  • Groupe de Physique des Solides, Universités Paris 6 et 7, UMR CNRS 7588, Campus Boucicaut, 140 rue de Lourmel, F-75015 Paris, France

Michel Alba

  • Laboratoire Léon Brillouin, UMR CEA-CNRS 12, CEA-Saclay, F-91191 Gif-sur-Yvette Cedex, France

Marc de Boissieu

  • Laboratoire de Thermodynamique et Physicochimie Métallurgiques, Institut National Polytechnique de Grenoble, Boîte Postale 75, F-38402 Saint Martin d’Hères, France

Marc Gailhanou

  • LURE, Batiment 209D, Université Paris–Sud, F-91405 Orsay Cedex, France

Michel Goldmann

  • Laboratoire des Objets Complexes et Interfaces d'Intérêt Biologique, Université Paris 5, FREE CNRS 2303, 45 rue des Saints Pères, Paris Cedex 6, France and LURE, Batiment 209D, Université Paris–Sud, F-91405 Orsay Cedex, France

  • *Electronic address: lacaze@gps.jussieu.fr

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Vol. 70, Iss. 1 — July 2004

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