Rheological Hysteresis in Soft Glassy Materials

Thibaut Divoux, Vincent Grenard, and Sébastien Manneville
Phys. Rev. Lett. 110, 018304 – Published 2 January 2013
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Abstract

The nonlinear rheology of a soft glassy material is captured by its constitutive relation, shear stress versus shear rate, which is most generally obtained by sweeping up or down the shear rate over a finite temporal window. For a huge amount of complex fluids, the up and down sweeps do not superimpose and define a rheological hysteresis loop. By means of extensive rheometry coupled to time-resolved velocimetry, we unravel the local scenario involved in rheological hysteresis for various types of well-studied soft materials. We introduce two observables that quantify the hysteresis in macroscopic rheology and local velocimetry, respectively, as a function of the sweep rate δt1. Strikingly, both observables present a robust maximum with δt, which defines a single material-dependent time scale that grows continuously from vanishingly small values in simple yield stress fluids to large values for strongly time-dependent materials. In line with recent theoretical arguments, these experimental results hint at a universal time scale-based framework for soft glassy materials, where inhomogeneous flows characterized by shear bands and/or pluglike flow play a central role.

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  • Received 17 July 2012

DOI:https://doi.org/10.1103/PhysRevLett.110.018304

© 2013 American Physical Society

Authors & Affiliations

Thibaut Divoux, Vincent Grenard, and Sébastien Manneville

  • Université de Lyon, Laboratoire de Physique, École Normale Supérieure de Lyon, CNRS UMR 5672, 46 Allée d’Italie, 69364 Lyon cedex 07, France

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Issue

Vol. 110, Iss. 1 — 4 January 2013

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