Nonlinear Nano-Optics: Probing One Exciton at a Time

N. H. Bonadeo, Gang Chen, D. Gammon, D. S. Katzer, D. Park, and D. G. Steel
Phys. Rev. Lett. 81, 2759 – Published 28 September 1998
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Abstract

Coherent nonlinear optical spectroscopy of individual excitons in GaAs quantum dots is demonstrated and shows strong similarities with atoms in their coherent optical interaction, unlike higher dimensional heterostructures. The nonlinear response is dominated by an incoherent contribution (saturation) and a coherent contribution (population pulsations) of the single dot and compares well with present theory. The data shows that energy relaxation and dephasing rates are comparable, reflecting the absence of significant pure dephasing, and also demonstrate the presence of interdot energy transfer.

  • Received 20 October 1997

DOI:https://doi.org/10.1103/PhysRevLett.81.2759

©1998 American Physical Society

Authors & Affiliations

N. H. Bonadeo1,2, Gang Chen1, D. Gammon3, D. S. Katzer3, D. Park3, and D. G. Steel2

  • 1The Harrison M. Randall Laboratory of Physics, The University of Michigan, Ann Arbor, Michigan 48109
  • 2The Center of Ultrafast Optical Science, The University of Michigan, Ann Arbor, Michigan 48109
  • 3Naval Research Laboratory, Washington, D.C. 20375

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Vol. 81, Iss. 13 — 28 September 1998

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