• Open Access

Role of electron scattering on the high-order harmonic generation from solids

Chang-Ming Wang, Nicolas Tancogne-Dejean, Massimo Altarelli, Angel Rubio, and Shunsuke A. Sato
Phys. Rev. Research 2, 033333 – Published 28 August 2020

Abstract

We extend the semiclassical trajectory description for the high-order harmonic generation (HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semiclassical trajectory model with a one-dimensional quantum mechanical simulation, we find that the multiplateau feature of the HHG spectrum is formed by Umklapp scattering under the electron-hole acceleration dynamics by laser fields. Furthermore, by tracing the scattered trajectories in real-space, the model fairly describes the emitted photon energy and the emission timing of the HHG even in the higher plateau regions. We further consider the loss of trajectories by scattering processes with a mean-free-path approximation and evaluate the HHG cutoff energy as a function of laser wavelength. As a result, we find that the trajectory loss by scattering causes the wavelength independence of the HHG from solids.

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  • Received 20 April 2020
  • Accepted 7 August 2020

DOI:https://doi.org/10.1103/PhysRevResearch.2.033333

Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. Open access publication funded by the Max Planck Society.

Published by the American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

Chang-Ming Wang1, Nicolas Tancogne-Dejean1, Massimo Altarelli1, Angel Rubio1,*, and Shunsuke A. Sato2,1,†

  • 1Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg, Germany
  • 2Center for Computational Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8577, Japan

  • *angel.rubio@mpsd.mpg.de
  • ssato@ccs.tsukuba.ac.jp

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Vol. 2, Iss. 3 — August - October 2020

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