Charge density wave modulation in superconducting BaPbO3/BaBiO3 superlattices

D. T. Harris, N. G. Campbell, C. Di, J.-M. Park, L. Luo, H. Zhou, G.-Y. Kim, K. Song, S.-Y. Choi, J. Wang, M. S. Rzchowski, and C. B. Eom
Phys. Rev. B 101, 064509 – Published 19 February 2020
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Abstract

The isotropic, nonmagnetic doped BaBiO3 superconductors maintain some similarities to high-Tc cuprates, while also providing a cleaner system for isolating charge density wave (CDW) physics that commonly competes with superconductivity. Artificial layered superlattices offer the possibility of engineering the interaction between superconductivity and CDW. Here we stabilize a low-temperature, fluctuating short-range CDW order by using artificially layered epitaxial (BaPbO3)3m/(BaBiO3)m (m=110 unit cells) superlattices that are not present in the optimally doped BaPb0.75Bi0.25O3 alloy with the same overall chemical formula. Charge transfer from BaBiO3 to BaPbO3 effectively dopes the former and suppresses the long-range CDW; however, as the short-range CDW fluctuations strengthen at low temperatures charge appears to localize and superconductivity is weakened. The monolayer structural control demonstrated here provides compelling implications to access controllable, local density wave orders absent in bulk alloys and manipulate phase competition in unconventional superconductors.

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  • Received 23 September 2018
  • Revised 27 December 2019
  • Accepted 23 January 2020

DOI:https://doi.org/10.1103/PhysRevB.101.064509

©2020 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

D. T. Harris1, N. G. Campbell2, C. Di3, J.-M. Park3, L. Luo3, H. Zhou4, G.-Y. Kim5, K. Song6, S.-Y. Choi5, J. Wang3, M. S. Rzchowski2, and C. B. Eom1,*

  • 1Department of Materials Science and Engineering, University of Wisconsin-Madison, Madison, Wisconsin 53706, USA
  • 2Department of Physics, University of Wisconsin-Madison, Madison, Wisconsin 53706, USA
  • 3Department of Physics and Astronomy and Ames Laboratory-U.S. DOE, Iowa State University, Ames, Iowa 50011, USA
  • 4Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439, USA
  • 5Department of Materials Science and Engineering, POSTECH, Pohang 37673, South Korea
  • 6Materials Modeling and Characterization Department, KIMS, Changwon 51508, South Korea

  • *eom@engr.wisc.edu

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Issue

Vol. 101, Iss. 6 — 1 February 2020

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