Abstract
We report on a comprehensive investigation of the effects of strain and film thickness on the structural and magnetic properties of epitaxial thin films of the prototypal compound by advanced x-ray scattering. We find that the thin films can be grown fully strained up to a thickness of 108 nm. By using x-ray resonant scattering, we show that the out-of-plane magnetic correlation length is strongly dependent on the thin film thickness, but independent of the strain state of the thin films. This can be used as a finely tuned dial to adjust the out-of-plane magnetic correlation length and transform the magnetic anisotropy from two-dimensional to three-dimensional behavior by incrementing film thickness. These results provide a clearer picture for the systematic control of the magnetic degrees of freedom in epitaxial thin films of and bring to light the potential for a rich playground to explore the physics of transition-metal compounds.
4 More- Received 22 September 2020
- Revised 4 November 2020
- Accepted 4 November 2020
DOI:https://doi.org/10.1103/PhysRevB.102.214402
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