Abstract
The structural properties of are studied using neutron diffraction, x-ray diffraction, and heat capacity measurements. The continuous orthorhombic-monoclinic structural phase transition in is suppressed linearly with Au substitution until a complete suppression of the structural phase transition occurs at the critical composition . Heat capacity measurements at low temperatures indicate residual structural instability at . The instability is ferroelastic in nature, with density functional theory calculations showing negligible coupling to electronic states near the Fermi level. The data and calculations presented here are consistent with the zero temperature termination of a continuous structural phase transition suggesting that the series hosts an elastic quantum critical point.
- Received 4 August 2016
DOI:https://doi.org/10.1103/PhysRevLett.117.235701
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