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ALMA Observations of CO Emission from Luminous Lyman-break Galaxies at z = 6.0293–6.2037

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Published 2022 December 13 © 2022. The Author(s). Published by the American Astronomical Society.
, , Citation Yoshiaki Ono et al 2022 ApJ 941 74 DOI 10.3847/1538-4357/ac9ea6

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Abstract

We present our new Atacama Large Millimeter/submillimeter Array (ALMA) observations targeting CO(6–5) emission from three luminous Lyman-break galaxies (LBGs) at zspec = 6.0293–6.2037 found in the Subaru/Hyper Suprime-Cam survey, whose [O iii] 88 μm and [C ii] 158 μm emissions have been detected with ALMA. We find a marginal detection of the CO(6–5) line from one of our LBGs, J0235–0532, at the ≃4σ significance level and obtain upper limits for the other two LBGs, J1211–0118 and J0217–0208. Our z = 6 luminous LBGs are consistent with the previously found correlation between the CO luminosity and the infrared luminosity. The unique ensemble of the multiple far-infrared emission lines and underlying continuum fed to a photodissociation region model reveals that J0235–0532 has a relatively high density of hydrogen nuclei nH that is comparable to those of low-z (U)LIRGs, quasars, and Galactic star-forming regions with high nH values, while the other two LBGs have lower nH consistent with local star-forming galaxies. By carefully taking account of various uncertainties, we obtain constraints on total gas mass and gas surface density from their CO luminosity measurements. We find that J0235–0532 is located below the Kennicutt–Schmidt (KS) relation, comparable to the z = 5.7 LBG, HZ10, previously detected with CO(2–1). Combined with previous results for dusty starbursts at similar redshifts, the KS relation at z = 5–6 is on average consistent with the local one.

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1. Introduction

Constraining the properties of molecular gas in galaxies across cosmic time is important for understanding galaxy formation and evolution (see the reviews of Carilli & Walter 2013; Tacconi et al. 2020). Although star formation proceeds through the conversion of molecular hydrogen, H2, into stars, it is difficult to directly detect emission from H2 in molecular clouds due to the lack of a permanent dipole moment and the high temperatures necessary to excite even the lowest transitions. 19 Instead, emission lines from rotational transitions of carbon monoxide, CO, are often employed to trace cold molecular gas in galaxies that is responsible for star formation activities.

Searches for CO line emission at z ≳ 3 have mainly focused on the most luminous sources such as quasars (e.g., Bertoldi et al. 2003; Walter et al. 2003; Maiolino et al. 2007; Weiß et al. 2007; Wang et al. 2013) and dusty starburst galaxies (e.g., Neri et al. 2003; Greve et al. 2005; Bothwell et al. 2013; Riechers et al. 2013; Weiß et al. 2013; Aravena et al. 2016; Zavala et al. 2018). For example, Riechers et al. (2010) have detected CO(2–1), CO(5–4), and CO(6–5) emission in a z = 5.3 dusty star-forming galaxy (SFG), AzTEC-3, and revealed a large molecular gas reservoir, maintaining its intense starburst with ≳ 1000 M yr−1. Another high-z example is a dusty SFG at z = 5.7, CRLE, whose CO(2–1) as well as [C ii] 158 μm and [N ii] 205 μm emissions have been detected in Pavesi et al. (2018), showing a large molecular gas reservoir with an intense starburst of ≃ 1500 M yr−1.

In contrast, little progress has been made for high-z normal SFGs such as Lyman-break galaxies (LBGs), which are more representative of the high-z galaxy population. Although a handful of CO detections have been reported in mostly lensed LBGs at z ∼ 3 (e.g., Baker et al. 2004; Ginolfi et al. 2017), to date only a few CO detections from normal SFGs at z > 3 have been reported: i.e., luminous LBGs, LBG-1 20 and HZ10, 21 at z = 5.3–5.7 (Pavesi et al. 2019; see also Riechers et al. 2014) and a likely damped Lyα absorber host, Serenity-18, at z = 5.9 (D'Odorico et al. 2018). CO lines from normal SFGs at z > 3 are typically too faint to allow for an investigation of the galaxy properties related to molecular gas components at high redshifts (e.g., Hashimoto et al. 2022), such as the gas surface density, the gas mass fraction, and the gas depletion time, and comparison with the Kennicutt–Schmidt (KS) relation (Schmidt 1959; Kennicutt 1998a), which are critically important for understanding the star formation process (e.g., Schinnerer et al. 2016; Kennicutt & De Los Reyes 2021) but have not yet been constrained well compared to those at lower redshifts.

In this study, we present our ALMA observations targeting CO(6–5) emission at ${\nu }_{\mathrm{CO}(6-5)}^{(\mathrm{rest})}=691.47\,\mathrm{GHz}$ in the rest frame, corresponding to the rest-frame wavelength of ${\lambda }_{\mathrm{CO}(6-5)}^{(\mathrm{rest})}=433.6$ μm, as well as dust continuum emission in three LBGs at z = 6 that have been identified in the Subaru/Hyper Suprime-Cam (HSC) survey (Aihara et al. 2018). Previous optical spectroscopic observations have detected Lyα emission from the three LBGs (Matsuoka et al. 2018), and subsequent ALMA observations have detected [O iii] 88 μm and [C ii] 158 μm emission lines in these galaxies (Harikane et al. 2020b).

This paper is outlined as follows. After introducing our three z = 6 luminous LBGs in Section 2, we describe our new ALMA observations and data reduction processes in Section 3. Our results for the CO emission and dust continuum emission from the three z = 6 luminous LBGs are presented in Section 4. We discuss their gaseous properties in Section 5 and present a summary in Section 6. Throughout this paper, we use magnitudes in the AB system (Oke & Gunn 1983) and assume a flat universe with Ωm = 0.3, ΩΛ = 0.7, and H0 = 70 km s−1 Mpc−1. In this cosmological model, an angular dimension of 1farcs0 corresponds to a physical dimension of 5.710 kpc at z = 6.0 (e.g., Equation (18) of Hogg 1999). We adopt the Chabrier (2003) initial mass function (IMF) with lower and upper mass cutoffs of 0.1 M and 100 M, respectively. Where necessary to convert star formation rates (SFRs) in the literature from the Salpeter (1955) IMF and the Kroupa (2001) IMF to the Chabrier IMF, we multiply by constant factors of αSC = 0.63 and αKC = 0.94 (= 0.63/0.67), respectively (Madau & Dickinson 2014).

2. Targets

To constrain the properties of molecular gas in z = 6 normal SFGs, we target three luminous LBGs at zspec = 6.029–6.204: J1211–0118, J0235–0532, and J0217–0208. Their basic properties reported in previous work are summarized in Table 1. These LBGs have been spectroscopically identified with Lyα emission (Matsuoka et al. 2018) and their [O iii] 88 μm, [C ii] 158 μm, and dust continuum emission have been observed with ALMA (Harikane et al. 2020b). Their total SFRs, SFRtot, have been estimated to be ∼100 M yr−1 as the sum of the dust-unobscured and dust-obscured SFRs based on the rest-frame ultraviolet (UV) and infrared (IR) continuum emission, SFRUV and SFRIR, respectively. These SFRs are estimated by using Equations (1) and (4) of Kennicutt (1998b) and considering the conversion factor from the Salpeter IMF to the Chabrier IMF. For details, see Appendix A. Because of their moderately high total SFRs, the CO emission line fluxes of our targets are expected to be high, if their molecular gas is not already depleted by recent star formation.

Table 1. Summary of the Properties of Our Targets

 J1211–0118J0235–0532J0217–0208
R.A.12:11:37.11202:35:42.41202:17:21.603
Decl.−01:18:16.500−05:32:41.623−02:08:52.778
MUV (mag)−22.8−22.8−23.3
LUV (1011 L)2.72.94.3
SFRUV (M yr−1)48 ± 348 ± 476 ± 4
re (kpc) a 1.200.97 b 0.57
EW${}_{0}^{\mathrm{Ly}\alpha }$ (Å)6.9 ± 0.841 ± 215 ± 1
βUV −2.0 ± 0.5−2.6 ± 0.6−0.1 ± 0.5
zsys 6.0293 ± 0.00026.0901 ± 0.00066.2037 ± 0.0005
L[O III]/L[C II] 3.4 ± 0.68.9 ± 1.76.0 ± 1.7

Notes. Most of the values presented in this table have been obtained in previous studies (Matsuoka et al. 2018; Harikane et al. 2020b).

a Half-light radius measured with the Subaru/HSC z-band images, which trace the rest UV continuum emission (Section 5.3). b This re value is measured with SExtractor, while the re values for the other targets are measured with GALFIT. This is because a numerical convergence problem may have occurred in the profile fitting with GALFIT for J0235–0532 (Section 5.3).

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Although their UV absolute magnitudes are MUV ≃ −23.0 mag, around which the luminosity functions of galaxies and active galactic nuclei (AGNs) are almost comparable (e.g., Ono et al. 2018), their rest UV spectra exhibit no clear signatures of AGNs such as broad Lyα or N v 1240 Å, suggesting that they are normal SFGs. Note that, because they are not located in a foreground galaxy cluster field or close to a foreground massive red galaxy, they are unlikely to be affected by strong lensing. Thus, they are great laboratories in which to investigate typical properties of high-z normal SFGs with no systematic uncertainties of lensing models.

3. ALMA Observations and Data Reduction

Our targets were observed during ALMA Cycle 7 with Band 3 between 2019 October 1 and 2019 November 12 (Project code: 2019.1.00156.S; PI: Y. Ono). The number of antennas used in the observations is 45. The antenna configurations were C43-3 for J0235–0532 and J0217–0208, and C43-4 for J1211–0118. The maximum baselines of C43-3 and C43-4 are 500.2 m and 2617.4 m, respectively. The minimum baseline of these configurations is 15.1 m. We used four spectral windows (SPWs) with 1.875 GHz bandwidths in the frequency division mode, yielding the total frequency coverage of 7.5 GHz. The velocity resolution was set to 3.9 MHz, which corresponds to about 10 km s−1. One of the SPWs was used for the CO(6–5) line and the others were used for the dust continuum. Note that CO(6–5) is the lowest CO excitation that can be observed for z = 6 galaxies with ALMA Bands 3–10. The details of the observations are presented in Table 2.

Table 2. Summary of Our ALMA Observations and Data

TargetDateConfigurationCentral Frequencies of SPWs tint PWV σcont Beam FWHMPA
 (YYYY-MM-DD) (GHz)(minutes)(mm)(μJy beam−1) (deg)
(1)(2)(3)(4)(5)(6)(7)(8)(9)
J1211–01182019-10-01C43-497.801, 99.488, 109.625, 111.50059.53.417.42farcs36 × 2farcs1559.56
J0235–05322019-11-12C43-396.964, 98.652, 108.825, 110.70091.75.59.73farcs17 × 2farcs72−72.15
J0217–02082019-11-12C43-395.434, 97.122, 107.325, 109.20072.65.27.43farcs18 × 2farcs7770.38

Note. (1) Target ID. (2) Observation date. (3) Antenna configuration. (4) Central frequencies of the four SPWs. (5) On-source integration time. (6) Precipitable water vapor. (7) The 1σ level of the continuum image. (8) The synthesized beam FWHM in units of arcsec × arcsec. (9) The position angle of the synthesized beam.

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We reduce the ALMA data by using the Common Astronomy Software Applications (CASA; McMullin et al. 2007) package 22 version 5.6.1. Using the CLEAN task, we produce continuum images and data cubes for our targets with the natural weighting. We apply a Gaussian taper with FWHM = 2farcs0 to improve the signal-to-noise ratio (S/N) for potentially existing low-surface-brightness emission. We adopt a pixel scale of 0farcs1 and a common spectral channel bin of about 60 km s−1. Table 2 presents the 1σ flux density levels and the spatial resolutions, and the synthesized beam position angles for the continuum images. Note that, although two of our targets were also observed with Northern Extended Millimeter Array (NOEMA), both show no detection, which is consistent with the ALMA results (Appendix B).

4. Results

4.1. CO(6–5)

For J0235–0532, the CO(6–5) emission line is marginally detected at the expected frequency from the systemic redshift, while for the other two targets, the CO(6–5) emission is not significantly detected. Figure 1 shows the ALMA spectra of our z = 6 luminous LBGs around their CO(6–5) emission line as expected from their systemic redshift measured by Harikane et al. (2020b) with the far-infrared (FIR) emission lines of [O iii] and [C ii]. The spectrum of J0235–0532 is extracted by placing a single beam aperture around the peak position of the CO emission in the CO(6–5) moment-zero map (velocity-integrated map; Figure 2), because the CO emission is not spatially resolved in the ALMA data. We fit Gaussian functions to the observed spectrum of J0235–0532 from 97.3 to 97.8 GHz and obtain the best-fit Gaussian function as presented in Figure 1. The integrated flux of this line calculated from the best-fit function is 0.0652 ± 0.0175 Jy km s−1, indicating that the CO(6–5) emission line of J0235–0532 shows a marginal detection at the ≃4σ significance level. Reassuringly the velocity width of the CO line is comparable to those of the previously detected [C ii] and [O iii] lines (Harikane et al. 2020b). Because the CO(6–5) is not significantly detected for J1211–0118 and J0217–0208 (Figures 1 and 2), we extract their spectra by placing a beam aperture based on the coordinates of their rest UV continuum emission. The upper limits of their CO(6–5) line fluxes are calculated from the square root of the sum of the squared flux density errors in the range of ±250 km s−1 around the expected CO(6–5) frequency from their systemic redshift. The range of ±250 km s−1 is comparable to twice the FWHM of their [O iii] and [C ii] emission lines (their FWHMs are about 170–370 km s−1; Table 1 of Harikane et al. 2020b). The integrated emission line flux or the upper limit for each target and the observed FWHM of the detected line are presented in Table 3.

Figure 1.

Figure 1. ALMA spectra of J1211–0118 (top), J0235–0532 (middle), and J0217–0208 (bottom) around the redshifted frequency of the CO(6–5) emission line (black histogram) extracted by placing a beam aperture (for details, see the text in Section 4.1). The dotted vertical line corresponds to the systemic redshift determined with the FIR emission lines of [O iii] and [C ii] (Harikane et al. 2020b). The red curve in the middle panel represents the best-fit Gaussian function to the CO(6–5) emission line.

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Figure 2.

Figure 2. Zeroth-moment images showing the integrated CO(6–5) flux densities of J1211–0118 (top), J0235–0532 (middle), and J0217–0208 (bottom). The synthesized beam is shown in the bottom left corner in each image. The size of each image is 30'' × 30''. The range of the color bar for the flux densities corresponds to ±3 times the standard deviation.

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Table 3. Summary of Our Observational Results

 J1211–0118J0235–0532J0217–0208
CO(6–5) integrated flux (Jy km s−1) <0.07130.0652 ± 0.0175 <0.0609
CO(6–5) FWHM (km s−1)237 ± 51
LCO(6−5) (107 L) <3.412.88 ± 0.773 <3.95
$L{{\prime} }_{\mathrm{CO}(6-5)}$ (109 K km s−1 pc2) <3.222.72 ± 0.73 <3.74
fν,430 μm (μJy) <52.3 <29.1 <22.1
LIR (1011 L) ${3.6}_{-1.9}^{+34.4}$ ${5.8}_{-5.8}^{+19.4}$ a ${2.0}_{-0.3}^{+5.9}$
Tdust (K) ${40}_{-14}^{+44}$ 50–80 (fixed) ${31}_{-9}^{+26}$
${f}_{\mathrm{CMB}}^{\mathrm{CO}(6-5)}$ 0.720.79–0.890.55
SFRIR (M yr−1) ${39}_{-21}^{+375}$ ${63}_{-63}^{+211}$ a ${22}_{-3}^{+64}$
SFRtot (M yr−1) ${88}_{-21}^{+375}$ ${112}_{-64}^{+211}$ ${98}_{-5}^{+65}$
Mgas (1010 M) <8.997.59 ± 4.74 <10.4
ΣSFR (M yr−1 kpc−2) ${9.6}_{-2.3}^{+41.5}$ ${18.9}_{-10.7}^{+35.6}$ ${48.2}_{-2.5}^{+31.6}$
Σgas (103 M pc−2) <9.912.8 ± 8.0 <5.1
fgas b <0.59 ${0.55}_{-0.23}^{+0.12}$ <0.46
tdep (Gyr) <1.02 ${0.68}_{-0.47}^{+0.90}$ <1.06

Notes. The upper limits are 3σ.

a These values are the 3σ upper limits when Tdust = 50 K, and the upper error takes into account the case when Tdust = 80 K. For details, see the text in Section 4.2. b The quoted uncertainties in the gas fraction do not include the systematic uncertainty associated with the stellar mass estimates.

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Figure 3 compares the ALMA spectra of our z = 6 luminous LBGs around the CO(6–5) emission line with those around the [O iii] and [C ii] emission lines. Although the S/N of the CO(6–5) line of J0235–0532 is not high, the redshifts based on the CO, [O iii], and [C ii] lines are broadly consistent with each other. Some previous studies have shown significant velocity shifts between [O iii] and [C ii] (e.g., BDF-3299 in Carniani et al. 2017; see Hashimoto et al. 2019; Bakx et al. 2020 as counterexamples); our results suggest that the velocity shift in J0235–0532, if any, is smaller than the previous results.

Figure 3.

Figure 3. ALMA spectra of J1211–0118 (left), J0235–0532 (center), and J0217–0208 (right) around CO(6–5), [O iii] 88 μm, and [C ii] 158 μm from top to bottom. The CO spectra are the same as the ones shown in Figure 1, but the velocity range is limited to [−1000 km s−1, 1000 km s−1]. The spectra for [O iii] 88 μm and [C ii] 158 μm have been obtained in Harikane et al. (2020b).

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Figure 4 presents the CO(6–5) emission contours of J0235–0532 with the Subaru HSC z-band image probing the rest-frame UV continuum emission. Although the positions of CO(6–5) and UV continuum appear to be slightly offset, this may be caused by the relatively low S/N of the CO emission. We estimate the uncertainties of the CO peak position by running a suite of Monte Carlo simulations in the same way as Harikane et al. (2020b). We add artificial noises to the actual data according to a Gaussian random distribution with a standard deviation equal to the 1σ noise of the data, and remeasure the peak positions one thousand times to estimate the uncertainties of the CO peak position. We find that the CO peak position is consistent with that of the UV continuum within the 2σ uncertainties. In Figure 4, we also present the [C ii] and [O iii] positions obtained in Harikane et al. (2020b), confirming that the CO peak position is also consistent with those of [C ii] and [O iii].

Figure 4.

Figure 4. CO(6–5) contours for J0235–0532. The red (blue) contours are multiples of 0.5σ (−0.5σ) starting at 2σ (−2σ). The synthesized beam is shown in the bottom left corner. The gray background is the Subaru HSC z-band image of J0235–0532 that captures the rest-frame UV continuum emission. The positions of the CO(6–5) and UV continuum emission are consistent within the large uncertainties (light red cross) estimated from the Monte Carlo simulations (for details, see the text in Section 4.1). The yellow and green crosses denote the positions of the [C ii] and [O iii] emission, respectively, and the sizes of the crosses are their uncertainties (Harikane et al. 2020b), which are also consistent with that of CO(6–5). The size of the image is 10'' × 10''.

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For a sanity check of the position of J0235–0532 in the HSC astrometry, which has been calibrated against the Pan-STARRS first data release (DR1) catalog (Chambers et al. 2016), we use nearby ($\lt 1^{\prime} $) bright stars whose positions are accurately measured in the Gaia early data release 3 (EDR3) catalog (Gaia Collaboration et al. 2016, 2021). 23 We confirm that the positional differences of the nearby bright stars between the HSC data and the Gaia EDR3 catalog are only within <0farcs01 with no systematic offsets, which is consistent with similar comparison results in previous work on a much larger scale (Section 6.3 of Aihara et al. 2019).

As mentioned above, the significance of the CO(6–5) line from J0235–0532 is only about 4σ. However, the observed CO peak position on the sky is consistent with that of the UV continuum, and the observed CO frequency is also in good agreement with those of the previously detected FIR emission lines; the probability of these events occurring simultaneously by chance is lower than the estimate above. We calculate the combined probability that these three events occur simultaneously by chance based on Fisher's method (Fisher 1970; see also Finke et al. 2015; Mulders et al. 2018; Kikuchihara et al. 2022; cf. Heard & Rubin-Delanchy 2018). First, the probability that the CO detection is a false positive can be calculated from the significance of the CO line from J0235–0532. We obtain a false-positive probability (p-value) of p1 ≃ 9.7 × 10−5, assuming that the flux measurement errors follow a Gaussian distribution. Second, the probability that the CO peak position is consistent with the previously detected source position can be calculated from the ratio of the area corresponding to the 2σ range to that of the obtained ALMA data. The p-value for this event is estimated to be p2 ≃ 7.3 × 10−4. Third, the probability that the detected line frequency coincides with those of the previously detected FIR lines can be calculated from the ratio of twice the FWHM frequency range to that of the four SPWs. The p-value for this event is estimated to be p3 ≃ 2.1 × 10−2. From these individual p-values, we calculate a test statistic (TS) for the combined probability,

Equation (1)

where k = 3 in this case. By comparing this TS with the χ2 distribution with 2k degrees of freedom, ${\chi }_{2k}^{2}$, we obtain a combined p-value pcom ≃ 3.4 × 10−7 from

Equation (2)

We then solve the equation

Equation (3)

to obtain an equivalent Gaussian standard deviation of S/Ncom ≃ 5.0 as the combined significance. In this paper, this signal for J0235–0532 is regarded as the CO(6–5) line. However, because the combined significance is still not very high, it is necessary to secure a firm detection of this CO line with follow-up observations.

Although the CO peak position is consistent with that of the UV continuum, the apparent offset (with large uncertainties) might indicate a hint of photoevaporation of photodissociation regions (PDRs; e.g., Carniani et al. 2017; Decataldo et al. 2017; Vallini et al. 2017). A partial displacement between the UV continuum tracing H ii regions and CO(6–5) emission tracing dense clumps within giant molecular clouds (GMCs; e.g., McKee & Ostriker 2007) is expected when PDRs are photoevaporated. (For details, see discussion in Vallini et al. 2017.) This scenario can be verified by observing the CO emission from J0235–0532 with a higher S/N and better resolution.

From the integrated CO(6–5) emission line flux, we obtain the CO(6–5) luminosity in units of L by using Equation (18) of Casey et al. (2014). We also calculate the CO(6–5) luminosity in units of K km s−1 pc2 defined by Equation (19) of Casey et al. (2014). These equations are presented in Appendix A. In these calculations, the effect of the cosmic microwave background (CMB) is taken into account by dividing the observed integrated flux by a factor of fCMB (da Cunha et al. 2013),

Equation (4)

where Bν is the Planck function, TCMB(z) = 2.73(1 + z) K is the temperature of the CMB, and Texc is the excitation temperature of the CO(6–5) transition. Assuming local thermal equilibrium (LTE), Texc is equal to the kinetic temperature of the gas, Tkin, and then to the dust temperature, Tdust, i.e., Texc = Tkin = Tdust. 24 Here we use Tdust estimated in Section 4.2. The obtained CO luminosities or upper limits, as well as the fCMB values, are presented in Table 3. 25 Note, as a caveat, that this prescription assumes a uniform kinetic temperature for CO- and dust continuum-emitting regions. However, in reality, PDRs have a kinetic temperature profile that depends on the radiation field and the gas density. If the kinetic temperature of the CO-emitting regions is higher than adopted here, Texc would be higher and thus fCMB would be higher (Section 2.4 of Vallini et al. 2015; see also Section 4.3 of Vallini et al. 2018). In this sense, the da Cunha et al. (2013) prescription may provide a pessimistic estimate of the fraction of the intrinsic flux observed.

4.2. Dust Continuum Emission

The dust continuum emission from our z = 6 luminous LBGs at λobs ≃ 3 mm (λrest ≃ 430 μm) is not significantly detected. The 3σ upper limits of their dust continuum flux densities are 52.3 μJy for J1211–0118, 29.1 μJy for J0235–0532, and 22.1 μJy for J0217–0208. Their dust continuum emission maps are presented in Appendix C.

In order to characterize the properties of their dust continuum emission, we combine our ALMA results at λrest ≃ 430 μm with the results of Harikane et al. (2020b) at shorter wavelengths of λrest ≃ 90–160 μm, and fit modified blackbody spectral energy distributions (SEDs) to the observed flux densities by varying Tdust and LIR. We calculate the intrinsic dust continuum flux densities of a modified blackbody SED by using Equation (A5), and then obtain the expected dust continuum flux densities of the modified blackbody, ${f}_{\nu }^{(\exp )}$, from ${f}_{\nu }^{(\mathrm{int})}$ by considering the CMB heating and attenuation effects based on the prescription of da Cunha et al. (2013) in the same way as described in Section 4.1. In the dust continuum SED fitting, we require that Tdust be higher than the CMB temperature at the redshift of the galaxy (∼20 K at z ∼ 6).

Figure 5 shows the results of fitting the modified blackbody SED to the observed SEDs. For J1211–0118 and J0217–0208, modified blackbody SEDs fit well with the observed SEDs. The best-fit IR luminosities and dust temperatures are (LIR, Tdust) = (${3.6}_{-1.9}^{+34.4}\times {10}^{11}\,{L}_{\odot }$, ${40}_{-14}^{+44}$ K) for J1211–0118 and (${2.0}_{-0.3}^{+5.9}\times {10}^{11}\,{L}_{\odot }$, ${31}_{-9}^{+26}$ K) for J0217–0208, which are consistent with the results of Harikane et al. (2020b). Considering the large Tdust uncertainties, the reason why the CO emission lines are not detected for these targets may be that the CMB attenuation effect for these targets is relatively large (fCMB is small) due to low Tdust. Because our observations only add an upper limit to the observed SEDs on the longer wavelength side of the SED peak, the parameter constraints do not become stronger than the previous work. The two parameters of LIR and Tdust are still degenerate, which will be greatly improved if deep observations of the dust continuum emission at shorter wavelengths than the SED peak are conducted. Note that another method has been proposed recently to determine Tdust and the dust mass assuming dust to be in radiative equilibrium if the source size of dust continuum emission is obtained (Inoue et al. 2020). Alternatively, it would be possible to have independent estimates of LIR and Tdust, as well as the dust mass, based on the dust continuum and [C ii] line luminosities by adopting the method recently presented in Sommovigo et al. (2021).

Figure 5.

Figure 5. Left: dust continuum SEDs of our z = 6 luminous LBGs, J1211–0118, J0235–0532, and J0217–0208 from top to bottom. The red arrows are the 3σ upper limits on the flux densities obtained in our ALMA observations. The black circles and downward arrows denote the observed flux densities and 3σ upper limits, respectively, obtained in Harikane et al. (2020b). The black solid curve indicates the best-fit modified blackbody and the gray shade corresponds to the 1σ uncertainties. Right: error contours for the two parameters LIR and Tdust in the modified blackbody fitting. The dark and light shades denote the 1σ and 2σ confidence regions, respectively. The black cross corresponds to the best-fit parameters.

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For J0235–0532, although the allowed parameter ranges are determined based on the upper limits of the flux densities, the constraints obtained on LIR and Tdust are not stringent. Following Harikane et al. (2020b), we adopt Tdust = 50 K for this galaxy without continuum detection as a fiducial value (see also Hashimoto et al. 2019) for comparisons with previous studies, which yields a 3σ upper limit of LIR < 5.8 × 1011 L. We also consider the case of a higher dust temperature of Tdust = 80 K as a systematic uncertainty. This is because J0235–0532 has the highest [O iii]/[C ii] luminosity ratio (Table 1), possibly suggesting a relatively high dust temperature. In fact, previous observations of nearby galaxies have shown that SFGs with higher [O iii]/[C ii] ratios tend to have higher Tdust values (Walter et al. 2018), although the [O iii]/[C ii] ratios of their SFGs are not as high as those of J0235–0532. More recently, dust continuum observations of a z = 8.31 galaxy with a similarly high [O iii]/[C ii] ratio, MACS0416-Y1, have suggested a possibility that its dust temperature may be extremely high, exceeding 80 K, although its physical origin is still under discussion (Bakx et al. 2020). One possible physical explanation for very high dust temperatures is that part of their dust is locked in molecular clouds and/or young star clusters that host active star formation. Based on hydrodynamic simulations, Behrens et al. (2018) have shown that, in such a situation, dust is heated by the strong interstellar radiation fields and can show a very high temperature, efficiently emitting FIR continuum, which can explain the high FIR luminosity without invoking mechanisms for massive dust production at high redshifts (see also, e.g., Arata et al. 2019; Sommovigo et al. 2020). The case of higher Tdust for J0235–0532 yields a more conservative upper limit of LIR < 2.5 × 1012 L (3σ).

In Figure 6, we compare the CO(6–5) and IR luminosities of our luminous LBGs at z = 6 with those of nearby sources at z < 0.1 (Liu et al. 2015) as well as dusty star-forming galaxies (DSFGs; Riechers et al. 2010; Strandet et al. 2017; D'Odorico et al. 2018; Apostolovski et al. 2019; Casey et al. 2019) and quasars (Wang et al. 2010, 2011, 2016; Venemans et al. 2017a; Carniani et al. 2019) at comparable redshifts of z ∼ 5–7 to our targets. For nearby sources, the correlation between CO and IR luminosities has been found over a wide luminosity range (Liu et al. 2015), which can be interpreted as an integrated KS relation because the CO and IR luminosities are correlated with gas mass and SFR, respectively (e.g., Magdis et al. 2017). We find that our result for J0235–0532, which is the only one of our targets showing CO(6–5) detection at the ≃4σ significance level, is broadly consistent with previous results owing to the relatively large uncertainty on the IR luminosity. For J1211–0118 and J0217–0208, whose CO emission is not detected, our results are also consistent with previous results. In other words, the obtained upper limits on CO luminosity for these two sources are not deep enough to know whether they deviate from the correlation between $L{{\prime} }_{\mathrm{CO}}$ and LIR seen in low-z sources or not, which can be distinguished by much deeper CO observations.

Figure 6.

Figure 6. IR luminosity integrated over the wavelength range of 8–1000 μm, LIR, vs. CO(6–5) luminosity in units of K km s−1 pc2, $L{{\prime} }_{\mathrm{CO}}$. The red circle is our ALMA result for a luminous LBG at z = 6, J0235–0532, whose CO(6–5) emission shows the 4σ significance level, with LIR and $L{{\prime} }_{\mathrm{CO}}$ in the case of Tdust = 50 K (Hashimoto et al. 2019; Harikane et al. 2020b). The upper error bar along the y-axis for J0235–0532 considers the case of a higher dust temperature of Tdust = 80 K. The red triangle and diamond are also our ALMA results for the other luminous LBGs at z = 6, J1211–0118 and J0217–0208, respectively, which show no significant CO(6–5) detection. The red arrows correspond to the 3σ upper limits. The orange squares are high-z DSFGs (Riechers et al. 2010; Strandet et al. 2017; D'Odorico et al. 2018; Apostolovski et al. 2019; Casey et al. 2019) and the magenta diamonds are high-z quasars (Wang et al. 2010, 2011, 2016; Venemans et al. 2017a; Carniani et al. 2019) at z ∼ 5–7. The black triangles are nearby galaxies, Seyfert galaxies, and (U)LIRGs at low redshifts (z < 0.1) compiled by Liu et al. (2015).

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Note that the excitation of the CO spectral line energy distribution (SLED) varies as a function of gas density, radiation field, Mach number within GMCs, and presence of shocks (e.g., Vallini et al. 2018; Pensabene et al. 2021), and thus the CO(6–5) emission line, which traces dense gas with critical density of ncrit = 2.9 × 105 cm−3, would trace a fraction of the total molecular gas, i.e., dense clumps within GMCs. Thus, the relation between $L{{\prime} }_{\mathrm{CO}(6-5)}$ and LIR would not be entirely related to the Mgas–SFR relation, and the interpretation as an integrated version of the KS relation could be partially hampered. In Sections 5.2 and 5.3, we convert $L{{\prime} }_{\mathrm{CO}(6-5)}$ to $L{{\prime} }_{\mathrm{CO}(1-0)}$ by adopting the average CO SLED for SFGs at lower redshifts to obtain the estimates of gas mass and gas surface density from $L{{\prime} }_{\mathrm{CO}(1-0)}$, and compare them with the KS relation found in the local universe, although the systematic uncertainties in such conversions are not small (Section 5.4).

5. Discussion

In this section, first we discuss physical origins for the relatively strong CO emission of J0235–0532 compared to the other two targets based on comparisons with a PDR model and previous results. Next, we derive the constraints on total gas mass from our CO results for the z = 6 luminous LBGs, and present comparisons of their gas surface densities with previous results. Finally, we caution that the obtained constraints on gas mass still have substantial systematic uncertainties. Note that we also present other gaseous properties of gas fraction and gas depletion timescale and compare them with previous results in Appendix D.

5.1. Physical Reasons for the Luminous CO(6–5) Emission in J0235–0532

In this study, we have observed CO(6–5) emission for the three luminous LBGs at z = 6 with comparable total SFRs of ∼100 M yr−1. As a result, CO(6–5) is marginally detected in J0235–0532 at the ≃4σ significance level, but not in the other two LBGs. In this section, we discuss physical reasons for this difference.

Because the [C ii] emission has also been detected for these LBGs in Harikane et al. (2020b), we calculate the line ratio of CO(6–5) to [C ii] as well as the ratio of the [C ii] to IR luminosity, which are useful for obtaining constraints on the physical properties of PDRs in galaxies such as the density of hydrogen nuclei, nH, and the incident far-ultraviolet (FUV) radiation field, UUV, with 6–13.6 eV based on comparisons with theoretical models for PDRs. For the PDR modeling, we use the Photodissociation Region Toolbox (PDRT; Kaufman et al. 1999, 2006; Pound & Wolfire 2008), 26 which calculates various line and continuum intensity ratios for combinations of nH and UUV by solving for the equilibrium chemistry, thermal balance, and radiation transfer through a PDR layer in a self-consistent way. Specifically, we use the wk2006 model of the PDRT with solar metallicity for comparisons with previous results.

Because the [C ii] emission comes from not only PDRs but also H ii regions, we need to subtract the contribution of [C ii] emission from H ii regions for comparisons with the results of the PDRT calculation. For this purpose, we refer to Figure 9 of Cormier et al. (2019), which presents the dependence of the fraction of [C ii] emission from H ii regions, ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$, on gas-phase metallicity (see also Figure 4 of Croxall et al. 2017; Sutter et al. 2019; Rybak et al. 2021; see also theoretical results such as Katz et al. 2017; Olsen et al. 2017; Ferrara et al. 2019; Pallottini et al. 2019). Based on analyses of interstellar medium absorption lines detected in the stacked spectrum of z ∼ 6 luminous LBGs with MUV ≃ −23 mag including one of our targets, J1211–0118, Harikane et al. (2020a) have found that their gas-phase metallicity is close to solar. 27 By combining these two previous results, ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ of our z = 6 luminous LBGs would be about ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}\simeq 0.3$. Because the observed ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ values have a scatter of ≃0.1–0.2, here we consider it as a systematic uncertainty. We also apply a factor-of-two correction for the observed CO flux considering line luminosity from both sides of each optically thick cloud for comparisons with the results of the PDRT calculation, as suggested by Kaufman et al. (1999) (see also Wang et al. 2016; Rybak et al. 2019; Shao et al. 2019).

Because the ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ values are correlated with the [C ii]/[N ii] 122 μm luminosity ratio as presented in Figure 10 of Cormier et al. (2019), we can also evaluate ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ from [C ii]/[N ii]. However, the [N ii] emission has not been detected in any of our targets (Harikane et al. 2020b), and the lower limits on the [C ii]/[N ii] ratios are not so stringent. Calculating the 3σ lower limits on the [C ii]/[N ii] ratios based on Table 1 of Harikane et al. (2020b), we obtain L[C II]/L[N II] > 0.36–2.3. We confirm that the expected ranges of the ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ values from the lower limits of the [C ii]/[N ii] ratios are consistent with those expected from the gas metallicity.

By taking account of these points, in the top left panel of Figure 7, we compare our ALMA results for LCO(6−5)/L[C II] versus L[C II]/LIR with the results of the PDRT calculation. Because the PDRT does not include the CMB temperature, the observed CO and IR luminosities are corrected for the CMB effect (Section 4). 28 In the same way as in Figure 6, we adopt Tdust = 50 K for J0235–0532 as a fiducial value and consider up to Tdust = 80 K as a systematic uncertainty, yielding a conservative lower limit of L[C II]/LIR. We find that the nH value of J0235–0532 is higher than those of J1211–0118 and J0217–0208. Because we only obtain the lower limit for the L[C II]/LIR ratio of J0235–0532 due to the nondetection of the dust continuum emission, it is unclear whether the incident FUV radiation is stronger in J0235–0532 than in the others or not.

Figure 7.

Figure 7. Top left: LCO(6−5)/L[C II] vs. L[C II]/LIR. The red circle is our ALMA result for a luminous LBG at z = 6 with ≃4σ CO(6–5) detection, J0235–0532, in the case of Tdust = 50 K, and the lower error bar along the x-axis considers the higher dust temperature case of Tdust = 80 K. The red triangle and diamond are also our ALMA results for the other luminous LBGs at z = 6, J1211–0118 and J0217–0208, respectively, which show no significant CO(6–5) detection. The red arrows correspond to the 3σ limits. The solid and dashed curves represent the theoretical calculations with the PDRT with constant densities of hydrogen nuclei, nH, in units of cm−3, and FUV (6–13.6 eV) radiation fields, UUV, in units of the average interstellar radiation field in the vicinity of the Sun, G0 = 1.6 × 10−3 erg s−1 cm−2 (Habing 1968), respectively. The blue arrow in the upper right corner represents the amount of shift when ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ increases by 0.1. The green arrow in the upper right corner shows the systematic uncertainties of the CMB effect on the [C ii] emission (Kohandel et al. 2019). Top right: LCO(1−0)/L[C II] vs. L[C II]/LIR. The orange squares denote LIRGs and ULIRGs (Rosenberg et al. 2015). The blue downward triangles and cyan triangles represent local SFGs and Galactic star-forming regions, respectively (Stacey et al. 1991). The magenta diamonds represent high-z quasars (Benford et al. 1999; Maiolino et al. 2005; Iono et al. 2006; Wagg et al. 2012, 2014; Leipski et al. 2013; Stefan et al. 2015; Wang et al. 2016; Venemans et al. 2017b; compiled by Shao et al. 2019). The solid and dashed curves are the same as in the left panel. In both panels, the CO line luminosities are multiplied by a factor of two as recommended by Kaufman et al. (1999) (for details, see the text in Section 5.1; see also Shao et al. 2019). Bottom: same as the top left panel, but with the colored shaded regions that roughly correspond to the low-z CO(1–0) results presented in the top right panel.

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For comparisons of the nH and UUV values of our z = 6 luminous LBGs with those of other sources at lower redshifts, in the top right panel of Figure 7, we show previous observation results for LCO(1−0)/L[C II] versus L[C II]/LIR of luminous infrared galaxies (LIRGs), ultraluminous infrared galaxies (ULIRGs; Rosenberg et al. 2015), quasars (Benford et al. 1999; Maiolino et al. 2005; Iono et al. 2006; Wagg et al. 2012, 2014; Leipski et al. 2013; Stefan et al. 2015; Wang et al. 2016; Venemans et al. 2017b; compiled by Shao et al. 2019), local SFGs such as spiral galaxies, and Galactic star-forming regions (Stacey et al. 1991), as well as the results of the PDRT model calculation. For easier comparison, the bottom panel of Figure 7 is the same as the top left panel but with the colored shaded regions that roughly correspond to the locations of low-z sources in the previous work with CO(1–0) observations shown in the top right panel. We find that the relatively high nH value of J0235–0532, nH ≳ 105 cm−3 depending on UUV, is consistent with those of LIRGs and ULIRGs with relatively low nH values in that population, as well as with those of quasars and Galactic star-forming regions with high nH and UUV values considering the case of high Tdust. We also find that J1211–0118 and J0217–0208, likely showing moderate UUV values with nH upper limits around 105 cm−3, are consistent with nuclear regions of local SFGs and Galactic star-forming regions with relatively low nH values.

It should be noted that there are two systematic uncertainties in this comparison. One is related to ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$. As mentioned above, the relation between ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ and metallicity has a scatter of about 0.1–0.2 (e.g., Figure 9 of Cormier et al. 2019). In our LCO(6−5)/L[C II] versus L[C II]/LIR figures, we show the blue arrow in the upper right corner that corresponds to the amount of shift when ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ is increased by 0.1. We confirm that this systematic uncertainty does not significantly affect the results. The other systematic uncertainty is the effect of the CMB on the [C ii] emission. As discussed in Section 6.1 of Harikane et al. (2020b), the [C ii] emission may also be affected by the CMB attenuation due to the high CMB temperature at z ∼ 6 (see also González-López et al. 2014; Lagache et al. 2018; Laporte et al. 2019). Figure 1 of Kohandel et al. (2019) shows the CMB suppression effect of the [C ii] emission with different gas temperatures as a function of gas number density. Although only upper limits are derived for nH of J1211–0118 and J0217–0208, with a conservative gas density value of 104 cm−3, we obtain the effect of the CMB on the [C ii] emission line flux of ${f}_{\mathrm{CMB}}^{[\mathrm{CII}]}=0.71$–0.86 at 30–40 K (Kohandel et al. 2019; see also Pallottini et al. 2015; Vallini et al. 2015), which is comparable to the dust temperature. If the gas density and/or the gas temperature is higher, then the CMB effect is smaller, suggesting that the impact of this systematic uncertainty is comparable to or smaller than that of the ${f}_{[{\rm{C}}\,{\rm\small{II}}]}^{(\mathrm{ion})}$ scatter.

There is another noticeable difference between J0235–0532 and the other two LBGs. J0235–0532 has the highest [O iii]/[C ii] luminosity ratio ([O iii]/[C ii] = 8.9 ± 1.7) among our targets, as shown in Figure 5 of Harikane et al. (2020b). In the first place, these three z = 6 LBGs have significantly higher [O iii]/[C ii] ratios than z ∼ 0 galaxies with comparable total SFRs. 29 Harikane et al. (2020b) have discussed the physical reason for this based on comparisons with the results of model calculations for both H ii regions and PDRs with CLOUDY (Ferland et al. 1998, 2017) and concluded that high ionization parameters and/or low PDR covering fractions can explain high-z galaxy results including the high [O iii]/[C ii] ratios and low L[C II]/SFR ratios. Harikane et al. (2020b) have also found that high nH, low C/O ratios, and the CMB attenuation effect can reproduce a part of the high-z galaxy results.

Because the CO emission originates from different regions from [O iii]-/[C ii]-emitting regions (e.g., Figure 31.2 of Draine 2011), it is difficult to make a direct comparison between our results and the results of Harikane et al. (2020b). The least we can say is that our results suggest a relatively high nH in PDRs of J0235–0532 compared to the other two LBGs, which would be consistent with the results of Harikane et al. (2020b), although in their study it is not enough to explain the high-z galaxy results. In addition, UUV of J0235–0532 may be higher than those of the other two LBGs, which would be consistent with the high [O iii]/[C ii] ratio and thus the relatively high ionization parameter, although deeper dust continuum observations are required for constraining L[C II]/LIR to reach a conclusion on this point.

Interestingly, this is in line with what is expected from theoretical models. The high-J CO lines trace regions of relatively high density more directly connected to star formation. At such a high density, the self-shielding effect prevents the dissociation of molecules and at the same time the high temperature produced by the strong UV radiation suggested from the high [O iii]/[C ii] ratio is expected to boost the high-J CO emission (Vallini et al. 2018). In this case, the dust temperature is also likely to be high (Behrens et al. 2018). In fact, the dust continuum is not detected only for J0235–0532, which is consistent with the possibility that the dust temperature of J0235–0532 may be very high. To confirm this picture, it would be interesting to carry out deep observations to detect high-J CO emission from SFGs with high [O iii]/[C ii] ratios and/or high Tdust, such as MACS1149-JD1 at z = 9.1096 ([O iii]/[C ii] ≳ 19; Hashimoto et al. 2018; Laporte et al. 2019), MACS0416-Y1 at z = 8.3118 ([O iii]/[C ii] = 8.6 ± 2.5 and Tdust > 80 K; Tamura et al. 2019; Bakx et al. 2020), and SXDF-NB1006-2 at z = 7.2120 ([O iii]/[C ii] ≳ 10; Inoue et al. 2016). Note that careful estimates of their [O iii]/[C ii] luminosity ratios have been provided recently by considering the surface brightness dimming effect (Carniani et al. 2020); they still show relatively high [O iii]/[C ii] values of 4.2 ± 1.4 for MACS1149-JD1, 8 ± 2 for MACS0416-Y1, and 4.3 ± 1.4 for SXDF-NB1006-2. We confirm that these sources also have high [O iii]/[C ii] surface brightness ratios (Vallini et al. 2021).

5.2. Constraints on Gas Mass

We constrain molecular gas masses in our z = 6 luminous LBGs based on our CO(6–5) results, although the systematic uncertainties are not small, particularly in the CO SLED, which has not been investigated well for SFGs at high redshifts. Here we present conservative constraints on molecular gas masses in our targets by taking account of such uncertainties and compare with previous results for lower-z sources.

The total gas mass for molecular clouds, Mgas, can be estimated from the CO(1–0) luminosity in units of K km s−1 pc2, $L{{\prime} }_{\mathrm{CO}(1-0)}$, by using Equation (4) of Solomon & Vanden Bout (2005),

Equation (5)

where αCO is the conversion factor from $L{{\prime} }_{\mathrm{CO}(1-0)}$ to Mgas. We assume a fixed value of αCO = 4.5 M (K km s−1 pc2)−1, 30 which is consistent with previous results for the Milky Way (Bolatto et al. 2013), z ∼ 1–2 SFGs (Daddi et al. 2010; Carilli & Walter 2013), and even an LBG at z = 5.7 (HZ10; Pavesi et al. 2019). 31 The $L{{\prime} }_{\mathrm{CO}(1-0)}$ values of our z = 6 luminous LBGs can be estimated from $L{{\prime} }_{\mathrm{CO}(6-5)}$ by using the average CO SLED for SFGs. Specifically, we assume that the integrated flux of CO(6–5) is comparable to that of CO(5–4), i.e., ICO(6−5)ICO(5−4), and adopt the average integral CO line flux ratio of ICO(5−4)/ICO(1−0) ≃ 5.8 ± 3.3, which is measured for z ∼ 1–2 SFGs (Daddi et al. 2015). The large uncertainty of ICO(5−4)/ICO(1−0) is estimated from the standard deviation of the integrated CO flux ratios of the z ∼ 1–2 SFGs reported in Daddi et al. (2015). 32 We then calculate $L{{\prime} }_{\mathrm{CO}(1-0)}$ 33 and obtain Mgas constraints as summarized in Table 3.

Note that Zanella et al. (2018) have reported a linear correlation between the [C ii] luminosity and the gas mass for z ∼ 2 SFGs and obtained a conversion factor from the [C ii] luminosity and the gas mass, ${\alpha }_{[{\rm{C}}\,{\rm\small{II}}]}=31\,{M}_{\odot }{L}_{\odot }^{-1}$. By adopting this conversion factor, we estimate the gas mass of J0235–0532 from the [C ii] luminosity to be only about 1.3 × 1010 M, which is significantly smaller than that obtained from the CO luminosity. This may suggest that the conversion factor α[C II] or αCO for high-z luminous LBGs is different from those at low redshifts, or that the CO SLED is different from those for z ∼ 1–2 SFGs, although it is difficult to clarify these possibilities with the currently available data. In this study, we adopt the estimates based on the CO luminosity, because it is more commonly used in previous studies and would thus be more appropriate for comparisons.

In Figure 8, we compare total SFRs and Mgas estimates of our z = 6 luminous LBGs with dusty starbursts and other SFGs over a wide range of redshifts from z ∼ 0 to z ∼ 6 (Béthermin et al. 2015; Scoville et al. 2016; Saintonge et al. 2017) including HZ10, LBG-1, AzTEC-3, and CRLE (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019). This figure should be interpreted as an integrated KS relation in a more direct sense than the LIR versus $L{{\prime} }_{\mathrm{CO}}$ plot presented as Figure 6 (Section 4.2). Following Kennicutt (1998a), we adopt the molecular gas mass as a proxy for the total gas mass for high-SFR sources including our z = 6 luminous LBGs, because such sources in the local universe show that the disks are molecular-dominated (Sanders & Mirabel 1996; see also Kennicutt & De Los Reyes 2021). Because we only obtain the upper limit of SFRIR for J0235–0532, we present the sum of SFRUV and the 2σ upper limit of SFRIR in the case of Tdust = 50 K as its total SFR, and consider the higher dust temperature up to Tdust = 80 K as well as the minimum SFR case of the SFRUV alone with no SFRIR in the relatively large error bars as systematic uncertainties. We find that our CO-based results for J0235–0532 are in broad agreement with SFGs at various redshifts with similar Mgas including HZ10 and LBG-1. J1211–0118 and J0217–0208 are consistent with the previous results with similar SFRs, although their Mgas values are upper limits.

Figure 8.

Figure 8. SFR vs. Mgas. The red circle is our ALMA result for a luminous LBG at z = 6 with ≃4σ CO(6–5) detection, J0235–0532, in the case of Tdust = 50 K and SFRtot = SFRUV + SFRIR,2σ . The error bar along the y-axis considers the case of a higher dust temperature of Tdust = 80 K and the minimum SFR case of SFRtot = SFRUV. Note that, although the intrinsic CO flux and thus the Mgas value become somewhat larger with a higher dust temperature, such a systematic uncertainty is much smaller than the uncertainty in the CO flux measurement. The red triangle and diamond are also our ALMA results for the other luminous LBGs at z = 6, J1211–0118 and J0217–0208, respectively, which show no significant CO(6–5) detection. The red arrows correspond to the 3σ limits. The blue squares represent the results of LBG-1 and HZ10 from left to right (Pavesi et al. 2019). The blue arrow represents the 3σ limit. The orange squares are the results of AzTEC-3 and CRLE from left to right (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019). The black filled downward triangles are the results of SFGs with Mstar > 3 × 1010 M at z ∼ 0–4 using stacked dust SEDs (Béthermin et al. 2015). The black open downward triangles show the results of SFGs with Mstar > 2 × 1010 M at z ∼ 1–6 based on submillimeter dust continuum measurements (Scoville et al. 2016). The black open triangles are the results for low-z galaxies at z = 0.01–0.05 (Saintonge et al. 2017).

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5.3. Kennicutt–Schmidt Relation

Although the currently available data for our z = 6 luminous LBGs do not resolve their internal structures in detail, we estimate their sizes to calculate their global SFR surface densities and gas surface densities for comparisons with the KS relation for the average surface densities of SFGs in the local universe.

The sizes of star-forming regions of our z = 6 luminous LBGs for calculating global SFR surface densities are measured with the HSC z-band images, which trace the rest UV continuum emission. We fit Sérsic profiles (Sersic 1968) to the observed surface brightness distributions by using GALFIT ver. 3.0.5 (Peng et al. 2002, 2010), 34 which convolves a galaxy model profile with a point-spread function (PSF) profile and optimizes the fitting parameters based on the Levenberg–Marquardt algorithm for χ2 minimization (e.g., Press et al. 1992). We use a PSF image for the position of each of our z = 6 luminous LBGs downloaded from the PSF picker website of the HSC survey. 35 The output parameters include the centroid coordinates of the objects, their total magnitude, the half-light radius along the semimajor axis, the axis ratio, and the position angle. The Sérsic index n is fixed at 1.0. 36 We calculate the circularized half-light radius, ${r}_{{\rm{e}}}=\sqrt{q}\,{r}_{{\rm{e}},\mathrm{maj}}$, where q is the axis ratio and re,maj is the half-light radius along the semimajor axis, because it is widely used in size measurements in previous high-z galaxy studies (e.g., Mosleh et al. 2012; Newman et al. 2012; Ono et al. 2013; Shibuya et al. 2015; Kawamata et al. 2018). The obtained re values are presented in Table 1.

Note that, for J0235–0532, the output axis ratio obtained with GALFIT is enclosed between star symbols, indicating that a numerical convergence issue may have occurred in the fitting for this particular source (for details, see Section 10 of the GALFIT user's manual). As an alternative method, for J0235–0532, we use SExtractor ver. 2.8.6 (Bertin & Arnouts 1996) 37 to calculate the observed half-light radius, ${r}_{{\rm{e}}}^{(\mathrm{obs})}$, by using circular apertures that contain half of the light from a galaxy, and correct it for the PSF broadening according to

Equation (7)

where rPSF is the half-light radius of the PSF image (e.g., Oesch et al. 2010; Holwerda et al. 2020; Bowler et al. 2021; Roberts-Borsani et al. 2022). For this PSF broadening correction, we use the PSF images downloaded from the PSF picker website. The obtained re value for J0235–0532 is also presented in Table 1. We also measure the half-light radii of J1211–0118 and J0217–0208 with SExtractor and confirm that the results are consistent with those obtained with GALFIT.

With the obtained re values, we define SFR surface density, ΣSFR, as the average SFR in a circular region whose half-light radius is re (Equation (A6)). The obtained ΣSFR values are listed in Table 3.

Because the resolution of our ALMA data is not high enough to estimate the sizes of CO-emitting regions, we calculate their gas surface densities by assuming that the sizes of CO-emitting regions are comparable to those of star-forming regions. In fact, Tacconi et al. (2013) have reported that molecular gas and UV/optical light distributions of z ∼ 1–2 SFGs show comparable sizes, in agreement with similar findings in z ∼ 0 SFGs (e.g., Regan et al. 2001; Leroy et al. 2008). With the re values obtained above, we define the gas surface density, Σgas, in a similar way to ΣSFR (Equation (A7)). 38 The obtained Σgas values are also presented in Table 3.

Figure 9 plots ΣSFR of our z = 6 luminous LBGs as a function of Σgas. For comparison, we also present normal spiral (disk) galaxies and starbursts in the local universe with the best-fit relation between their ΣSFR and Σgas (the KS relation; de los Reyes & Kennicutt 2019; Kennicutt & De Los Reyes 2021; see also Kennicutt 1998a), 39 as well as the z = 5.3–5.7 sources, HZ10, LBG-1, AzTEC-3, and CRLE (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019). We find that J0235–0532 and HZ10 are almost at the same position in this plane, located below the local KS relation, suggesting that J0235–0532 and HZ10 have very high gas surface densities with relatively low star formation efficiencies. We also find that J1211–0118 and J0217–0208 are consistent with the local KS relation, although their obtained Σgas values are upper limits. Note that in Figure 8 their data points are consistent with the integrated KS relation, while in Figure 9 they are below the local KS relation. The reason for this is that our z = 6 luminous LBGs have smaller gas-emitting regions and/or larger star-forming regions than those of local starbursts. In Figure 9, we confirm that the dusty starbursts at comparable redshifts, AzTEC-3 and CRLE, are located above the local KS relation. These results may indicate that the scatter of the KS relation is larger with increasing redshift, at least at large Σgas of ∼104 M pc−2, possibly suggesting that star formation in high-z galaxies with high Σgas is diverse, ranging from bursty to slow. However, the number of high-z data points is still limited; this needs to be examined by investigating more objects at high redshifts in the future. Averaging the four data points for the z = 5–6 galaxies of J0235–0532, HZ10, AzTEC-3, and CRLE, we find that the z = 5–6 KS relation at Σgas ∼ 104 M pc−2 on average is consistent with the KS relation in the local universe. Again, the number of high-z sources whose ΣSFR and Σgas are estimated is limited yet. It would be interesting to compare the observational results for a larger sample of high-z galaxies with those of theoretical studies in the future (e.g., Ferrara et al. 2019; Dubois et al. 2021).

Figure 9.

Figure 9. ΣSFR vs. Σgas. The red filled circle is our ALMA result for a luminous LBG at z = 6 with ≃4σ CO(6–5) detection, J0235–0532, in the case of Tdust = 50 K and SFRtot = SFRUV + SFRIR,2σ . The error bar along the y-axis considers the case of a higher dust temperature of Tdust = 80 K and the minimum SFR case of SFRtot = SFRUV. The red filled triangle and diamond are also our ALMA results for the other luminous LBGs at z = 6, J1211–0118 and J0217–0208, respectively, which show no significant CO(6–5) detection. The red arrows correspond to the 3σ limits. We also present the results for our z = 6 luminous LBGs adopting the CO SLED and αCO for Althaea for their total gas mass estimates, and the previously obtained [C ii] sizes as their gas sizes (red open circle: J0235–0532; red open triangle: J1211–0118; red open diamond: J0217–0208; for details, see Section 5.4). The blue squares represent the results of LBG-1 and HZ10 from left to right (Pavesi et al. 2019). Note that the data point of HZ10 is shifted by +0.1 dex along the x-axis for visibility. The blue arrow represents the 3σ limit. The orange squares are the results of AzTEC-3 and CRLE from left to right (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019). The brown star denotes the average of the four data points of J0235–0532, HZ10, AzTEC-3, and CRLE as the average KS relation at z = 5–6, although the number of high-z sources whose ΣSFR and Σgas are estimated is limited. The black open triangles and squares denote local spiral galaxies and starbursts compiled by de los Reyes & Kennicutt (2019) and Kennicutt & De Los Reyes (2021), respectively. The blue solid line corresponds to the KS relation, $\mathrm{log}{{\rm{\Sigma }}}_{\mathrm{SFR}}=(1.50\pm 0.02)\mathrm{log}{{\rm{\Sigma }}}_{\mathrm{gas}}-3.87\pm 0.04$ (Kennicutt & De Los Reyes 2021) and the blue shaded region represents the ΣSFR values that can be obtained when the two parameters of the KS relation change within the 2σ uncertainties. Note that the ΣSFR values in de los Reyes & Kennicutt (2019) and Kennicutt & De Los Reyes (2021) are corrected by a factor of αKC (Section 1) to consider the IMF difference (Table E1).

Standard image High-resolution image

Note that the re values measured in the rest UV continuum images are used in the calculations of both the SFR and gas surface densities for our z = 6 luminous LBGs. If their CO sizes are significantly larger than the rest UV sizes, the currently presented Σgas values correspond to the upper limits (e.g., Kaasinen et al. 2020). More quantitative discussion about this point is presented in Section 5.4. In order to obtain more accurate Σgas values with no such systematic uncertainties, high-resolution deep CO observations are necessary.

5.4. Systematic Uncertainties

In Sections 5.2 and 5.3, we obtain the total gas mass estimates for our z = 6 luminous LBGs based on our CO(6–5) observation results by carefully considering the uncertainties suggested from the previous observation results, and discuss the KS relation. However, we caution that the gas mass estimates have substantial systematic uncertainties.

One is the CO SLED uncertainty. In our discussion above, we adopt the previously observed CO SLED results for z ∼ 1–2 SFGs and consider the significant amount of scatter seen in observations of individual objects (Daddi et al. 2015). However, our z = 6 luminous LBGs may be experiencing more bursty star formation with higher gas density and thus the CO SLED could be more excited. For example, previous CO observations of nearby starbursts have revealed that their integrated CO flux ratios are about ICO(6−5)/ICO(1−0) ≃ 8–20 (Figure 1 of Mashian et al. 2015). 40 Based on the ALMA Spectroscopic Survey in the Hubble Ultra Deep Field (ASPECS), Boogaard et al. (2020) have shown that SFGs at $\left\langle z\right\rangle =2.5$ have higher CO excitation than those at $\left\langle z\right\rangle =1.2$ as well as the results of Daddi et al. (2015), suggesting the increased CO excitation at higher redshifts (e.g., Figure 7 of Boogaard et al. 2020). Theoretically, Vallini et al. (2018) have developed a semianalytical model for GMCs where the CO lines are excited, and postprocessed a state-of-the-art zoom-in cosmological simulation of a main-sequence galaxy at z = 6, Althaea, with Mstar ≈ 1010 M and SFR ≈ 100 M yr−1 (Pallottini et al. 2017), which is in line with the nature of the galaxies discussed in this paper, showing that the CO SLED of Althaea has a peak at around the upper-state rotational quantum number of Jup ≃ 6. Specifically, Althaea has CO luminosities of about $L{{\prime} }_{\mathrm{CO}(1-0)}\simeq {10}^{9.2}$ K km s−1 pc2 and $L{{\prime} }_{\mathrm{CO}(6-5)}\simeq {10}^{8.9}$ K km s−1 pc2, yielding the CO luminosity ratio of $L{{\prime} }_{\mathrm{CO}(1-0)}/L{{\prime} }_{\mathrm{CO}(6-5)}\simeq 2.0$. In contrast, the CO luminosity ratio that we have adopted in our discussion above is $L{{\prime} }_{\mathrm{CO}(1-0)}/L{{\prime} }_{\mathrm{CO}(6-5)}=6.2\pm 3.5$ (Equation (6) in Section 5.2). Although their theoretical result is just for one z = 6 galaxy, their upcoming results with the SERRA simulation show that the physical mechanisms exciting the CO SLED (i.e., high density and high turbulence) are common in more than 100 high-z galaxies (A. Pallottini 2022, in preparation; see also Pallottini et al. 2019). If the CO SLEDs of our z = 6 luminous LBGs are similar to that of Althaea, the gas mass estimates become lower by a factor of about 1/3. This should be examined by observing several CO emission lines with different excited states from high-z SFGs.

Another systematic uncertainty comes from the CO-to-H2 conversion factor, αCO. In our discussion above, we adopt the fixed value of αCO = 4.5 M (K km s−1 pc2)−1, which is consistent with the previous observational results such as for the Milky Way, z ∼ 1–2 SFGs, and HZ10 at z = 5.7 (Daddi et al. 2010; Bolatto et al. 2013; Carilli & Walter 2013; Pavesi et al. 2019). However, it is known that the CO-to-H2 conversion factor becomes smaller in galaxies with more active star formation. In fact, LIRGs and ULIRGs show low CO-to-H2 conversion factors of αCO ≃ 0.8 M (K km s−1 pc2)−1 (Downes & Solomon 1998), which is often adopted in previous studies of high-z dusty starbursts (e.g., Greve et al. 2005; Riechers et al. 2010; Aravena et al. 2016; see also Wagg et al. 2009). Our z = 6 luminous LBGs may also have small αCO values compared to the adopted one. From a theoretical point of view, Vallini et al. (2018) have shown that the simulated z = 6 galaxy Althaea has a small αCO value of αCO = 1.5 M (K km s−1 pc2)−1 (see their Figure 12; see also Narayanan et al. 2012). If our z = 6 luminous LBGs have small αCO values comparable to Althaea, the gas mass estimates based on the CO(6–5) results are further reduced by a factor of 1/3. Interestingly, if we adopt the CO SLED and αCO for Althaea, the obtained gas mass estimate for J0235–0532 from CO(6–5) is consistent with that obtained from the [C ii] luminosity (Section 5.2).

Furthermore, in the calculations of the gas surface densities of our z = 6 luminous LBGs, we assume that the sizes of CO-emitting regions are comparable to those of star-forming regions, which is also a source of systematic uncertainties. As mentioned in Section 5.3, some previous observational studies for z ∼ 0–2 SFGs have shown that this is the case (Regan et al. 2001; Leroy et al. 2008; Tacconi et al. 2013), while some other studies have shown that the gas sizes are larger. For our z = 6 luminous LBGs, Carniani et al. (2020) have reported their [C ii] sizes (FWHMs along the major axis) in their Table A1. If the [C ii] sizes are comparable to those of CO-emitting regions and the CO luminosities are comparable to the current measurements, the gas sizes become larger by about a factor of 3, and thus Σgas becomes smaller by about a factor of 1/10. This can be tested by deep observations of low-J CO emission, which better traces the molecular gas distribution and the total gas mass.

If we adopt the CO SLED and αCO for Althaea for total gas mass estimates, and use the previously obtained [C ii] sizes as their gas sizes, then the estimated gas surface densities of our z = 6 luminous LBGs become smaller by about two orders of magnitude than presented in Figure 9. Figure 9 adds this possibility on the ΣSFR–Σgas plot. In this case, our z = 6 luminous LBGs are located above the KS relation, which means that they are experiencing bursty star formation. Because their [O iii]/[C ii] ratios are relatively high compared to local galaxies with similar total SFRs (Section 5.1), this interpretation may be physically more reasonable (Vallini et al. 2021; see also Ferrara et al. 2019). This issue is expected to be clarified by future follow-up observations.

6. Summary

In this study, we have presented our ALMA observation results for the CO(6–5) and dust continuum emission from the three luminous LBGs with −22.8 > MUV > −23.3 mag at zspec = 6.0293–6.2037 identified in the Subaru/HSC survey. Their [O iii] 88 μm and [C ii] 158 μm emission lines have been detected in the previous work (Harikane et al. 2020b). Our main results are as follows.

  • 1.  
    Out of the three z = 6 luminous LBGs, we have marginal detection of the CO(6–5) emission at the ≃4σ significance level at the expected frequency from the previously detected [O iii] 88 μm and [C ii] 158 μm lines.
  • 2.  
    No dust continuum emission at λrest ≃ 430 μm is significantly detected for our z = 6 luminous LBGs. By combining the obtained upper limits with the previous results at shorter wavelengths of λrest ≃ 90–160 μm, we have updated the dust continuum SED fitting analyses, and confirmed that our obtained constraints on LIR and Tdust are consistent with the previous results of Harikane et al. (2020b).
  • 3.  
    We have compared the CO(6–5) and IR luminosities of our z = 6 luminous LBGs with those of other sources over a wide range of redshifts in the literature by taking into account the CMB effect and the Tdust uncertainty. We have found that our z = 6 luminous LBGs are consistent with the previous results owing to the relatively large uncertainties.
  • 4.  
    By comparing the LCO/L[C II] and L[C II]/LIR ratios of our z = 6 luminous LBGs with previous observations and results of the PDR model calculation, we have found that J0235–0532 has a relatively high nH value comparable to those of low-z LIRGs and ULIRGs, as well as those of quasars and Galactic star-forming regions with high nH and UUV values. We have also found that J1211–0118 and J0217–0208 have lower nH values consistent with local SFGs and Galactic star-forming regions with relatively low nH values.
  • 5.  
    By carefully taking into account the systematic uncertainties in the CO SLED, Mgas constraints for our z = 6 luminous LBGs have been obtained based on our CO(6–5) observation results. We have found that J0235–0532 is in broad agreement with SFGs at various redshifts with similar Mgas in the literature, including the z = 5.3–5.7 SFGs of HZ10 and LBG-1. We have also found that the Mgas upper limits for J1211–0118 and J0217–0208 are consistent with the previous results with comparable SFRs.
  • 6.  
    We have calculated the global SFR and gas surface densities of our z = 6 luminous LBGs based on the total SFR and Mgas constraints, with the sizes of star-forming regions measured in the HSC images capturing the rest UV continuum emission. We have found that J0235–0532 is at almost the same position as HZ10 on the ΣSFR–Σgas plane, located slightly below the local KS relation, indicating that J0235–0532 and HZ10 have high gas surface densities with relatively low star formation efficiencies. We have also found that the upper limits of Σgas for J1211–0118 and J0217–0208 are consistent with the local KS relation. Because the dusty starbursts at similar redshifts, AzTEC-3 and CRLE, are located above the local KS relation, our results and the previous results may suggest that the scatter of the KS relation increases with increasing redshift at least at large Σgas. In addition, the average z = 5–6 KS relation at Σgas ∼ 104 M pc−2 is in agreement with the local KS relation. However, the number of high-z sources whose ΣSFR and Σgas have been estimated is still limited; the high-z KS relation needs to be determined with better accuracy to discuss the average and the scatter by investigating more objects at high redshifts in the future.
  • 7.  
    We caution that the obtained gas mass estimates for our z = 6 luminous LBGs have substantial systematic uncertainties such as the CO SLED, the CO-to-H2 conversion factor αCO, and gas sizes. If we adopt the CO SLED and the αCO value suggested by the state-of-the-art zoom-in cosmological simulation and the gas sizes measured with [C ii] emission, the gas surface densities estimated for our z = 6 luminous LBGs can become larger by about two orders of magnitude, which opens up two conflicting possibilities regarding their location below or above the KS relation. This situation should be clarified by pursuing further CO observations of high-z SFGs.

We acknowledge the constructive comments and helpful suggestions from the anonymous referee that helped us to improve the manuscript. We appreciate the support of the staff at the ALMA Regional Center, especially Kazuya Saigo, for giving us helpful advice on analyzing the ALMA data. We are grateful to the staff of the IRAM facilities, especially Michael Bremer and Melanie Krips, for helping us to reduce the NOEMA data. We also thank Daizhong Liu for sharing their data with us, and Marc Pound and Mark Wolfire for their helpful advice on using the results of the PDRT calculation.

This paper made use of the following ALMA data: ADS/JAO.ALMA#2019.1.00156.S and ADS/JAO.ALMA#2017.1.00508.S. ALMA is a partnership of ESO (representing its member states), NSF (USA) and NINS (Japan), together with NRC (Canada), MOST and ASIAA (Taiwan), and KASI (Republic of Korea), in cooperation with the Republic of Chile. The Joint ALMA Observatory is operated by ESO, AUI/NRAO and NAOJ.

This work is based on observations carried out under project numbers W18FB and S19DK with the IRAM NOEMA Interferometer. IRAM is supported by INSU/CNRS (France), MPG (Germany) and IGN (Spain).

The Hyper Suprime-Cam (HSC) collaboration includes the astronomical communities of Japan and Taiwan, and Princeton University. The HSC instrumentation and software were developed by the National Astronomical Observatory of Japan (NAOJ), the Kavli Institute for the Physics and Mathematics of the Universe (Kavli IPMU), the University of Tokyo, the High Energy Accelerator Research Organization (KEK), the Academia Sinica Institute for Astronomy and Astrophysics in Taiwan (ASIAA), and Princeton University. Funding was contributed by the FIRST program from the Japanese Cabinet Office, the Ministry of Education, Culture, Sports, Science and Technology (MEXT), the Japan Society for the Promotion of Science (JSPS), Japan Science and Technology Agency (JST), the Toray Science Foundation, NAOJ, Kavli IPMU, KEK, ASIAA, and Princeton University.

This paper makes use of software developed for the Large Synoptic Survey Telescope. We thank the LSST Project for making their code available as free software at http://dm.lsst.org.

This paper is based in part on data collected at the Subaru Telescope and retrieved from the HSC data archive system, which is operated by Subaru Telescope and Astronomy Data Center (ADC) at NAOJ. Data analysis was in part carried out with the cooperation of Center for Computational Astrophysics (CfCA), NAOJ.

The Pan-STARRS1 Surveys (PS1) and the PS1 public science archive have been made possible through contributions by the Institute for Astronomy, the University of Hawaii, the Pan-STARRS Project Office, the Max Planck Society and its participating institutes, the Max Planck Institute for Astronomy, Heidelberg, and the Max Planck Institute for Extraterrestrial Physics, Garching, The Johns Hopkins University, Durham University, the University of Edinburgh, the Queen's University Belfast, the Harvard-Smithsonian Center for Astrophysics, the Las Cumbres Observatory Global Telescope Network Incorporated, the National Central University of Taiwan, the Space Telescope Science Institute, the National Aeronautics and Space Administration under grant No. NNX08AR22G issued through the Planetary Science Division of the NASA Science Mission Directorate, the National Science Foundation grant No. AST-1238877, the University of Maryland, Eotvos Lorand University (ELTE), the Los Alamos National Laboratory, and the Gordon and Betty Moore Foundation.

This work has made use of data from the European Space Agency (ESA) mission Gaia (https://www.cosmos.esa.int/gaia), processed by the Gaia Data Processing and Analysis Consortium (DPAC, https://www.cosmos.esa.int/web/gaia/dpac/consortium). Funding for the DPAC has been provided by national institutions, in particular the institutions participating in the Gaia Multilateral Agreement.

This work was partially performed using the computer facilities of the Institute for Cosmic Ray Research, The University of Tokyo. This work was supported by the World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan, as well as KAKENHI grant Nos. 15K17602, 15H02064, 17H01110, 17H01114, 19K14752, 20H00180, and 21H04467 through the Japan Society for the Promotion of Science (JSPS). This work was partially supported by the joint research program of the Institute for Cosmic Ray Research (ICRR), University of Tokyo. A.F., A.P., and L.V. acknowledge support from the ERC Advanced Grant INTERSTELLAR H2020/740120. A.F. acknowledges generous support from the Carl Friedrich von Siemens-Forschungspreis der Alexander von Humboldt-Stiftung Research Award. A.K.I. and Y.S. are supported by NAOJ ALMA Scientific Research Grant Code 2020-16B. T.H. was supported by Leading Initiative for Excellent Young Researchers, MEXT, Japan (HJH02007) and KAKENHI (20K22358).

Software: IRAF (Tody 1986, 1993), 41 SAOImage DS9 (Joye & Mandel 2003), Numpy (Harris et al. 2020), Matplotlib (Hunter 2007), Scipy (Virtanen et al. 2020), Astropy (Astropy Collaboration et al. 2013, 2018), 42 and Ned Wright's Javascript Cosmology Calculator (Wright 2006), 43 CASA (McMullin et al. 2007), GILDAS (Guilloteau & Lucas 2000; Pety 2005; Gildas Team 2013), SExtractor (Bertin & Arnouts 1996), GALFIT (Peng et al. 2002, 2010).

Appendix A: Standard Equations

In this appendix, we present the standard equations used in this study for reference.

In Section 2, we estimate SFRs for our z = 6 luminous LBGs by using Equation (1) of Kennicutt (1998b),

Equation (A1)

where Lν is the rest UV luminosity density in units of erg s−1 Hz−1, and Equation (4) of Kennicutt (1998b), 44

Equation (A2)

where LIR is the IR luminosity integrated over the wavelength range 8–1000 μm in units of erg s−1. We multiply by αSC to convert from the Salpeter IMF to the Chabrier IMF.

In Section 4.1, from the integrated CO(6–5) emission line flux, we obtain the CO(6–5) luminosity in units of L by using Equation (18) of Casey et al. (2014),

Equation (A3)

where ICO is the integrated CO flux in units of Jy km s−1 and DL(z) is the luminosity distance in Mpc. We also calculate the CO(6–5) luminosity in units of K km s−1 pc2 defined as Equation (19) of Casey et al. (2014),

Equation (A4)

where ${\nu }_{\mathrm{CO}}^{(\mathrm{obs})}={\nu }_{\mathrm{CO}}^{(\mathrm{rest})}/(1+z)$.

In Section 4.2, the intrinsic dust continuum flux densities of a modified blackbody SED at a given observed frequency νobs are calculated from (e.g., Ouchi et al. 1999; Ono et al. 2014)

Equation (A5)

where B(ν, T) is the Planck function and ν0 = νobs(1 + z). We assume a spectral index of βd = 1.5, which is consistent with local measurements for SFGs (e.g., Dunne & Eales 2001; Gordon et al. 2010; Casey 2012) and often adopted in previous high-z studies (e.g., Casey et al. 2014; Franco et al. 2020; Harikane et al. 2020b; see also Sugahara et al. 2021; Schouws et al. 2022). Harikane et al. (2020b) have confirmed that this assumption does not significantly affect the fitting results of the other parameters for our targets.

In Section 5.3, we define SFR surface density, ΣSFR, in units of M yr−1 kpc−2 as the average SFR in a circular region whose half-light radius is re,

Equation (A6)

The multiplicative factor of 1/2 is applied because the SFR is estimated from the total luminosity while the area is calculated with the half-light radius (e.g., Hathi et al. 2008; Tacconi et al. 2013; Decarli et al. 2016). In a similar way, we define the gas surface density as

Equation (A7)

Appendix B: NOEMA Observations

In addition to the ALMA observations described in Section 3, two of our targets, J1211–0118 and J0217–0208, were also observed with NOEMA using 9–10 antennas between 2019 January 20 and 2019 August 15 (Proposal IDs: W18FB and S19DK; PI: Y. Ono). The antenna configurations were A and D, i.e., the most extended and the compact configurations, respectively. We used the NOEMA receiver 1 to observe the CO(6–5) emission as well as the dust continuum emission from the two LBGs. The total observing times were 5.5 hr for J1211–0118 and 13.9 hr for J0217–0208. All the NOEMA data are reduced using the GILDAS software. 45 The 1σ flux density levels for the continuum images are 13.8 μJy beam−1 for J1211–0118 and 13.9 μJy beam−1 for J0217–0208. The NOEMA data show no significant detection of either dust continuum emission or CO emission, which is consistent with the ALMA results (Section 4.2).

Appendix C: Dust Continuum Emission Maps

In Figure 10, we present the dust continuum emission maps at λobs ≃ 3 mm (λrest ≃ 430 μm) obtained with ALMA for our z = 6 luminous LBGs. For J0235–0532, the ±300 km s−1 range around the CO(6–5) line is removed.

Figure 10.

Figure 10. Dust continuum emission maps for our z = 6 luminous LBGs, J1211–0118, J0235–0532, and J0217–0208 from left to right. The red contours are continuum emission at λrest ≃ 430 μm drawn at 1σ intervals from 1.5σ. Although the dust continuum of J0235 and J0217 may show a ∼2σ signal, in this paper we conservatively use their 3σ upper limits. The blue lines represent negative contours from −1.5σ at 1σ intervals. The red ellipses at the lower left corner denote the ALMA synthesized beams. The gray backgrounds are the Subaru HSC z-band images that capture the rest UV continuum emission from our targets. The size of each image is 10'' × 10''.

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Appendix D: Extra Results Related to Gas Masses

In addition to the comparisons between gas masses and SFRs as well as the Kennicutt–Schmidt relation shown in Section 5, in this appendix we present the gas fractions and gas depletion timescales for comparisons with previous results, although the systematic uncertainties on these estimates are also not small as discussed in Section 5.4.

D.1. Gas Fraction

We constrain gas fractions for our z = 6 luminous LBGs. The gas fraction is defined as

Equation (D1)

where Mstar is the stellar mass. For our z = 6 luminous LBGs, Mstar can be roughly estimated from MUV by using the relation between Mstar and MUV for SFGs at similar redshifts, e.g., Equation (2) of Shibuya et al. (2015),

Equation (D2)

where βSC = 1/1.64 ≃ 0.61 is the factor to convert from Mstar with the Salpeter (1955) IMF to that with the Chabrier (2003) IMF (Madau & Dickinson 2014; see also Table E1). We present the obtained fgas constraints in Table 3. Note that our fgas constraints do not include the systematic uncertainty in the stellar mass estimates from the UV luminosity, which is about ±0.5 dex due to differences in stellar population properties such as star formation history (Shibuya et al. 2015). For more robust discussion, deep rest-frame optical data that can probe the stellar continuum emission are required.

In Figure 11, we present fgas of our z = 6 luminous LBGs with those of lower-z SFGs (Béthermin et al. 2015; Scoville et al. 2016; Saintonge et al. 2017) as well as the z = 5.3–5.7 sources, HZ10, LBG-1, AzTEC-3, and CRLE (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019) as a function of total SFR. We find that J0235–0532 has a comparable gas fraction to lower-z SFGs with similar SFRs. We also find that the obtained upper limits on the gas fractions of J1211–0118 and J0217–0208 are consistent with lower-z SFGs with similar SFRs. Compared to HZ10, the gas fraction of J0235–0532 is consistent owing to the large uncertainties, while those of J1211–0118 and J0217–0208 are significantly lower, although their total SFRs are comparable.

Figure 11.

Figure 11. Gas fraction, fgas = Mgas/(Mgas + Mstar), as a function of SFR. The red circle is our ALMA result for a luminous LBG at z = 6 with ≃4σ CO(6–5) detection, J0235–0532, in the case of Tdust = 50 K and SFRtot = SFRUV + SFRIR,2σ . The error bar along the y-axis considers the case of a higher dust temperature of Tdust = 80 K and the minimum SFR case of SFRtot = SFRUV. The red triangle and diamond are also our ALMA results for the other luminous LBGs at z = 6, J1211–0118 and J0217–0208, respectively, which show no significant CO(6–5) detection. The red arrows correspond to the 3σ limits. The blue squares represent the results of LBG-1 and HZ10 from left to right (Pavesi et al. 2019). The blue arrow represents the 3σ limit. The orange squares are the results of AzTEC-3 and CRLE from left to right (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019). The black filled downward triangles are the results of SFGs with Mstar > 3 × 1010 M at z ∼ 0–4 using stacked dust SEDs (Béthermin et al. 2015). The black open downward triangles show the results of SFGs with Mstar > 2 × 1010 M at z ∼ 1–6 based on submillimeter dust continuum measurements (Scoville et al. 2016). The black open triangles are the results for low-z galaxies at z = 0.01–0.05 (Saintonge et al. 2017).

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D.2. Evolution of the Gas Depletion Timescale

Figure 12 shows the gas depletion timescale, tdep = Mgas/SFR, as a function of redshift. For comparison, we also present the results for the four z = 5.3–5.7 sources of HZ10, LBG-1, AzTEC-3, and CRLE (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019), the average results for z = 4.4–5.9 LBGs with Mstar = 108.4−11 M obtained in the ALMA Large Program to Investigate [C ii] at Early Times (ALPINE; Dessauges-Zavadsky et al. 2020), and other SFGs including dusty starbursts over a wide range of redshifts (Béthermin et al. 2015; Aravena et al. 2016; Schinnerer et al. 2016; Scoville et al. 2016; Magdis et al. 2017; Saintonge et al. 2017).

Figure 12.

Figure 12. Redshift evolution of the gas depletion time, tdep = Mgas/SFR. The red circle is our ALMA result for a luminous LBG at z = 6 with ≃4σ CO(6–5) detection, J0235–0532, in the case of Tdust = 50 K and SFRtot = SFRUV + SFRIR,2σ . The error bar along the y-axis for J0235–0532 considers the case of a higher dust temperature of Tdust = 80 K and the minimum SFR case of SFRtot = SFRUV. The red triangle and diamond are also our ALMA results for the other luminous LBGs at z = 6, J1211–0118 and J0217–0208, respectively, which show no significant CO(6–5) detection. The red arrows correspond to the 3σ limits. The blue squares represent the results of LBG-1 and HZ10 from left to right (Pavesi et al. 2019). The blue arrow represents the 3σ limit. The orange squares are the results of AzTEC-3 and CRLE from left to right (Riechers et al. 2010, 2014; Pavesi et al. 2018; see also Pavesi et al. 2019). The blue filled triangles show the average results of z = 4.4–5.9 LBGs with Mstar = 108.4−11 M obtained in the ALPINE survey (Dessauges-Zavadsky et al. 2020), where Mgas are estimated from the [C ii] luminosities. The black filled triangles denote the results based on CO observations of z ∼ 3 LBGs (Magdis et al. 2017). The black filled downward triangles are the results of SFGs with Mstar > 3 × 1010 M using stacked dust SEDs (Béthermin et al. 2015). The black open downward triangles show the results of SFGs with Mstar > 2 × 1010 M based on submillimeter dust continuum measurements (Schinnerer et al. 2016; Scoville et al. 2016). The black open squares are the results for lensed/unlensed dusty starburst sources compiled by Aravena et al. (2016). The dashed and dotted lines correspond to the curves of tdep ∝ (1 + z)−1.0 and tdep ∝ (1 + z)−1.5 (e.g., Davé et al. 2012; Tacconi et al. 2013), which are normalized to the typical gas depletion time of 1.5 Gyr observed for local galaxies (Leroy et al. 2008; Bigiel et al. 2011; Saintonge et al. 2011, 2012; see also Saintonge et al. 2013).

Standard image High-resolution image

As expected from Figure 8, tdep of J0235–0532 is comparable to those of lower-z SFGs at z ∼ 2–3. Based on previous results for lower-z SFGs, Tacconi et al. (2013) have suggested a redshift dependence of the gas depletion timescale in the form of tdep ∝ (1 + z)−1.0, which is shallower than what is expected if tdep is proportional to the dynamical timescale, tdep ∝ (1 + z)−1.5 (Davé et al. 2011, 2012; see also Saintonge et al. 2013). Our results for J0235–0532 show that the tdep value is likely to be larger than expected from the previously reported redshift dependences. For the other two z = 6 luminous LBGs, J1211–0118 and J0217–0208, we have obtained upper limits on their tdep, indicating that their tdep values can be significantly shorter than that for J0235–0532. In other words, there is a possibility that tdep values of high-z SFGs are not necessarily as large as those of lower-z SFGs, suggesting that J0235–0532 may be an outlier with large tdep. Similar arguments can be made at slightly lower redshifts based on the results of HZ10 and LBG-1 as well as the ALPINE results. Because the previous results for lower-z SFGs show a large scatter of tdep, it would be interesting to investigate a typical tdep value by observing more high-z SFGs with better sensitivities in future studies to characterize the typical star formation properties in high-z SFGs.

Appendix E: Adopted IMFs in the Literature

In this paper, we have adopted the Chabrier (2003) IMF with lower and upper mass cutoffs of 0.1 M and 100 M, respectively, as described in Section 1. However, some previous studies have adopted different IMFs, and corrections for IMF differences are required when comparing physical quantities related to IMFs such as SFR and Mstar. For convenience in such purposes, Table E1 summarizes the IMFs adopted in the previous studies whose SFR or Mstar estimates are used for comparisons with our results. Where necessary to convert SFR and Mstar values in the literature, we use constant factors of αSC, αKC, and βSC, as described in Section 1 and Appendix D.1.

Table E1. IMFs Adopted in the Previous Studies

Previous StudyIMF
Riechers et al. (2014)Chabrier (2003)
Béthermin et al. (2015)Chabrier (2003)
Shibuya et al. (2015)Salpeter (1955)
Scoville et al. (2016)Chabrier (2003)
Aravena et al. (2016)Chabrier (2003)
Schinnerer et al. (2016)Chabrier (2003)
Magdis et al. (2017)Chabrier (2003)
Saintonge et al. (2017)Chabrier (2003)
Pavesi et al. (2018)Chabrier (2003)
de los Reyes & Kennicutt (2019)Kroupa (2001)
Pavesi et al. (2019)Chabrier (2003)
Harikane et al. (2020b)Chabrier (2003)
Dessauges-Zavadsky et al. (2020)Chabrier (2003)
Kennicutt & De Los Reyes (2021)Kroupa (2001)

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Footnotes

  • 19  

    Specifically, the two lowest H2 rotational transitions have upper level energies of h ν/kB = 510 and 1015 K above ground (Dabrowski 1984), and the lowest H2 vibrational transition is even more difficult to excite, corresponding to h ν/kB = 6471 K (Bolatto et al. 2013).

  • 20  

    LBG-1 is also named HZ6 (Capak et al. 2015).

  • 21  

    CRLE is serendipitously discovered in Atacama Large Millimeter/submillimeter Array (ALMA) observations targeting HZ10 (Pavesi et al. 2018).

  • 22  
  • 23  
  • 24  

    Note that, even in the case of non-LTE, if the gas temperature and density are relatively high, the CMB effect for the CO(6–5) line is comparable to that in the LTE case (see the non-LTE example with Tkin = 40 K and the number density of H2 molecules ${n}_{{{\rm{H}}}_{2}}={10}^{4.2}$ cm−3 in Figure 10 of da Cunha et al. 2013; cf. Figure 6 of da Cunha et al. 2013).

  • 25  

    Because no dust continuum is detected in J0235–0532 in our data and the previous data (Harikane et al. 2020b), the obtained constraint on Tdust is not stringent. We thus consider the Tdust uncertainty when we obtain the uncertainties of the physical quantities of J0235–0532 that are related to Tdust such as the IR luminosity and the CO luminosity. For details, see Section 4.2.

  • 26  
  • 27  

    This result is consistent with our use of the wk2006 model of the PDRT with solar metallicity.

  • 28  

    Although we compare the observed results corrected for the CMB effect with the results of the PDRT calculation, the PDRT calculation with the consideration of the CMB effect may change the shape of the diagnostic (M. Wolfire 2022, private communication). We need to check this point when the theoretical models are updated in the future.

  • 29  

    It should be noted that the [O iii]/[C ii] luminosity ratio of some high-z galaxies can be overestimated because the [C ii]-emitting region of ALMA-detected high-z galaxies is typically about 2–3 times more extended than the [O iii] and UV continuum-emitting regions (Carniani et al. 2020; see also Fujimoto et al. 2019, 2020; Herrera-Camus et al. 2021). To capture the extended [C ii] emission, Harikane et al. (2020b) have calculated the total line fluxes with a large (2'' radius) aperture (see their Sections 4.1 and 6.1). Recently, Vallini et al. (2021) have proposed that the [O iii]/[C ii] surface brightness ratio is also useful to overcome this issue. We confirm that our z = 6 luminous LBGs also have high [O iii]/[C ii] surface brightness ratios and J0235–0532 shows the highest value among them (Vallini et al. 2021; see also Carniani et al. 2020).

  • 30  

    The systematic uncertainties related to this conversion factor are discussed in Section 5.4.

  • 31  

    Pavesi et al. (2019) have estimated the total gas mass by subtracting the contribution of stars and dark matter masses from the dynamical mass measured with the significantly detected [C ii] line, and obtained the αCO value from the ratio of the estimated total gas mass to the CO luminosity. They have found that the obtained αCO value is ${\alpha }_{\mathrm{CO}}={4.2}_{-1.7}^{+2}\,{M}_{\odot }$ (K km s−1 pc2)−1, which is consistent with that of the Milky Way, although the uncertainty is not small.

  • 32  

    Although here we consider the standard deviation of the previous observation results, the uncertainties of the CO SLEDs may be much larger. The details of this point are presented in Section 5.4.

  • 33  

    The CO(1–0) luminosity is calculated from

    Equation (6)

    where ${\nu }_{\mathrm{CO}(1-0)}^{(\mathrm{rest})}=115.27\,\mathrm{GHz}$.

  • 34  
  • 35  
  • 36  

    We confirm that the obtained sizes show little difference if we use n = 1.5.

  • 37  
  • 38  

    Note that our assumption that these sizes are comparable may cause a systematic uncertainty, because some previous results indicate that the sizes of CO-emitting regions are not comparable to those in the rest UV/optical, as described in the last paragraph of this section and discussed more quantitatively in Section 5.4.

  • 39  

    Because the Kroupa IMF is adopted in de los Reyes & Kennicutt (2019) and Kennicutt & De Los Reyes (2021) as listed in Table E1, their ΣSFR values are corrected by a factor of αKC (Section 1).

  • 40  

    In their paper, the CO fluxes, fCO, have units of W m−2; for comparison we use the following conversion obtained from Equation (A3):

    Equation (8)

    Here we do not consider the AGNs and Seyfert galaxies presented in their figure.

  • 41  

    IRAF is distributed by the National Optical Astronomy Observatory, which is operated by the Association of Universities for Research in Astronomy (AURA) under a cooperative agreement with the National Science Foundation.

  • 42  
  • 43  
  • 44  

    Note that this conversion does not take into account the contribution from old stars whose emission is absorbed by dust and reradiated in the IR spectral range, although it would not be significant for high-z LBGs. In order to estimate SFRs from IR continuum luminosities by appropriately considering the contribution from old stars, one needs a more general recipe such as the one derived by Inoue et al. (2000; see also Hirashita et al. 2003).

  • 45  
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10.3847/1538-4357/ac9ea6